Pushing the limit of 3d transition metal-based layered oxides that use both cation and anion redox for energy storage

M Zhang, DA Kitchaev, Z Lebens-Higgins… - Nature Reviews …, 2022 - nature.com
Intercalation chemistry has dominated electrochemical energy storage for decades, and
storage capacity worldwide has now reached the terawatt-hour level. State-of-the-art …

Sodium transition metal oxides: the preferred cathode choice for future sodium-ion batteries?

Q Liu, Z Hu, W Li, C Zou, H Jin, S Wang… - Energy & …, 2021 - pubs.rsc.org
The exploration of next-generation sodium-ion batteries (SIBs) is a worldwide concern to
replace the current commercial lithium-ion batteries, mitigating the increasing exhaustion of …

[PDF][PDF] Progress on modification strategies of layered lithium-rich cathode materials for high energy lithium-ion batteries

H Lu, R Hou, S Chu, H Zhou, S Guo - Acta Phys.-Chim. Sin, 2023 - whxb.pku.edu.cn
High-performance rechargeable lithium-ion batteries have been widely used in portable
electronic devices, electric vehicles and other fields of electrochemical energy storage …

Correlative operando microscopy of oxygen evolution electrocatalysts

JT Mefford, AR Akbashev, M Kang, CL Bentley… - Nature, 2021 - nature.com
Transition metal (oxy) hydroxides are promising electrocatalysts for the oxygen evolution
reaction,–. The properties of these materials evolve dynamically and heterogeneously with …

First-cycle voltage hysteresis in Li-rich 3d cathodes associated with molecular O2 trapped in the bulk

RA House, GJ Rees, MA Pérez-Osorio, JJ Marie… - Nature Energy, 2020 - nature.com
Li-rich cathode materials are potential candidates for next-generation Li-ion batteries.
However, they exhibit a large voltage hysteresis on the first charge/discharge cycle, which …

Decoupling the roles of Ni and Co in anionic redox activity of Li-rich NMC cathodes

B Li, Z Zhuo, L Zhang, A Iadecola, X Gao, J Guo… - Nature Materials, 2023 - nature.com
Abstract Li [Li x Ni y Mn z Co1− x− y− z] O2 (lithium-rich NMCs) are benchmark cathode
materials receiving considerable attention due to the abnormally high capacities resulting …

Origin and regulation of oxygen redox instability in high-voltage battery cathodes

X Liu, GL Xu, VSC Kolluru, C Zhao, Q Li, X Zhou, Y Liu… - Nature Energy, 2022 - nature.com
Oxygen redox at high voltage has emerged as a transformative paradigm for high-energy
battery cathodes such as layered transition-metal oxides by offering extra capacity beyond …

The role of O2 in O-redox cathodes for Li-ion batteries

RA House, JJ Marie, MA Pérez-Osorio, GJ Rees… - Nature Energy, 2021 - nature.com
The energy density of Li-ion batteries can be improved by storing charge at high voltages
through the oxidation of oxide ions in the cathode material. However, oxidation of O2 …

Delocalized electron holes on oxygen in a battery cathode

RA House, GJ Rees, K McColl, JJ Marie… - Nature Energy, 2023 - nature.com
Oxide ions in transition metal oxide cathodes can store charge at high voltage offering a
route towards higher energy density batteries. However, upon charging these cathodes, the …

A Mechanistic Insight into the Oxygen Redox of Li‐Rich Layered Cathodes and their Related Electronic/Atomic Behaviors Upon Cycling

S Kang, D Choi, H Lee, B Choi, YM Kang - Advanced Materials, 2023 - Wiley Online Library
Li‐rich cathodes are extensively investigated as their energy density is superior to Li
stoichiometric cathode materials. In addition to the transition metal redox, this intriguing …