Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …
carbon neutral through an alternative electrical approach to the energy-intensive …
Gas diffusion electrodes, reactor designs and key metrics of low-temperature CO2 electrolysers
CO2 emissions can be recycled via low-temperature CO2 electrolysis to generate products
such as carbon monoxide, ethanol, ethylene, acetic acid, formic acid and propanol. In recent …
such as carbon monoxide, ethanol, ethylene, acetic acid, formic acid and propanol. In recent …
Room-temperature photosynthesis of propane from CO2 with Cu single atoms on vacancy-rich TiO2
Photochemical conversion of CO2 into high-value C2+ products is difficult to achieve due to
the energetic and mechanistic challenges in forming multiple CC bonds. Herein, an efficient …
the energetic and mechanistic challenges in forming multiple CC bonds. Herein, an efficient …
Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling
Electroreduction of carbon dioxide (CO2) into multicarbon products provides possibility of
large-scale chemicals production and is therefore of significant research and commercial …
large-scale chemicals production and is therefore of significant research and commercial …
Electrocatalytic CO2-to-C2+ with Ampere-Level Current on Heteroatom-Engineered Copper via Tuning *CO Intermediate Coverage
An ampere-level current density of CO2 electrolysis is critical to realize the industrial
production of multicarbon (C2+) fuels. However, under such a large current density, the poor …
production of multicarbon (C2+) fuels. However, under such a large current density, the poor …
Rational design of electrocatalytic carbon dioxide reduction for a zero-carbon network
Electrocatalytic CO2 reduction has attracted much attention for its potential application in
CO2 mitigation and fuel production. During the past two decades, the electrocatalytic …
CO2 mitigation and fuel production. During the past two decades, the electrocatalytic …
Identification of Cu(100)/Cu(111) Interfaces as Superior Active Sites for CO Dimerization During CO2 Electroreduction
The electrosynthesis of valuable multicarbon chemicals using carbon dioxide (CO2) as a
feedstock has substantially progressed recently but still faces considerable challenges. A …
feedstock has substantially progressed recently but still faces considerable challenges. A …
Localized Alkaline Environment via In Situ Electrostatic Confinement for Enhanced CO2-to-Ethylene Conversion in Neutral Medium
Electrocatalytic CO2 reduction reaction (CO2RR) is one of the most promising routes to
facilitate carbon neutrality. An alkaline electrolyte is typically needed to promote the …
facilitate carbon neutrality. An alkaline electrolyte is typically needed to promote the …
Highly selective and productive reduction of carbon dioxide to multicarbon products via in situ CO management using segmented tandem electrodes
Electrochemical CO2 reduction provides a promising route to the sustainable generation of
valuable chemicals and fuels. Tandem catalysts enable sequential CO2-to-CO and CO-to …
valuable chemicals and fuels. Tandem catalysts enable sequential CO2-to-CO and CO-to …
Tunable CO2 electroreduction to ethanol and ethylene with controllable interfacial wettability
The mechanism of how interfacial wettability impacts the CO2 electroreduction pathways to
ethylene and ethanol remains unclear. This paper describes the design and realization of …
ethylene and ethanol remains unclear. This paper describes the design and realization of …