Molecular chirality and its monitoring by ultrafast x-ray pulses
Major advances in X-ray sources including the development of circularly polarized and
orbital angular momentum pulses make it possible to probe matter chirality at …
orbital angular momentum pulses make it possible to probe matter chirality at …
Simulating coherent multidimensional spectroscopy of nonadiabatic molecular processes: From the infrared to the x-ray regime
Crossings of electronic potential energy surfaces in nuclear configuration space, known as
conical intersections, determine the rates and outcomes of a large class of photochemical …
conical intersections, determine the rates and outcomes of a large class of photochemical …
Roadmap on quantum light spectroscopy
S Mukamel, M Freyberger, W Schleich… - Journal of physics B …, 2020 - iopscience.iop.org
Conventional spectroscopy uses classical light to detect matter properties through the
variation of its response with frequencies or time delays. Quantum light opens up new …
variation of its response with frequencies or time delays. Quantum light opens up new …
Ultrafast spectroscopy of photoactive molecular systems from first principles: Where we stand today and where we are going
Computational spectroscopy is becoming a mandatory tool for the interpretation of the
complex, and often congested, spectral maps delivered by modern non-linear multi-pulse …
complex, and often congested, spectral maps delivered by modern non-linear multi-pulse …
Ultrafast X-ray probes of elementary molecular events
Elementary events that determine photochemical outcomes and molecular functionalities
happen on the femtosecond and subfemtosecond timescales. Among the most ubiquitous …
happen on the femtosecond and subfemtosecond timescales. Among the most ubiquitous …
Monitoring molecular nonadiabatic dynamics with femtosecond X-ray diffraction
K Bennett, M Kowalewski… - Proceedings of the …, 2018 - National Acad Sciences
Ultrafast time-resolved X-ray scattering, made possible by free-electron laser sources,
provides a wealth of information about electronic and nuclear dynamical processes in …
provides a wealth of information about electronic and nuclear dynamical processes in …
Probing electronic fluxes via time-resolved x-ray scattering
The current flux density is a vector field that can be used to describe theoretically how
electrons flow in a system out of equilibrium. In this work, we unequivocally demonstrate that …
electrons flow in a system out of equilibrium. In this work, we unequivocally demonstrate that …
[HTML][HTML] Monitoring nonadiabatic avoided crossing dynamics in molecules by ultrafast X-ray diffraction
We examine time-resolved X-ray diffraction from molecules in the gas phase which undergo
nonadiabatic avoided-crossing dynamics involving strongly coupled electrons and nuclei …
nonadiabatic avoided-crossing dynamics involving strongly coupled electrons and nuclei …
X-ray sum frequency diffraction for direct imaging of ultrafast electron dynamics
X-ray diffraction from molecules in the ground state produces an image of their charge
density, and time-resolved x-ray diffraction can thus monitor the motion of the nuclei …
density, and time-resolved x-ray diffraction can thus monitor the motion of the nuclei …
Monitoring vibronic coherences and molecular aromaticity in photoexcited cyclooctatetraene with an X-ray probe: a simulation study
Understanding conical intersection (CI) dynamics and subsequent conformational changes
is key for exploring and controlling photo-reactions in aromatic molecules. Monitoring of their …
is key for exploring and controlling photo-reactions in aromatic molecules. Monitoring of their …