Deconvolving contributions to decoherence in molecular electron spin qubits: a dynamic ligand field approach
R Mirzoyan, NP Kazmierczak… - Chemistry–A European …, 2021 - Wiley Online Library
In the past decade, transition metal complexes have gained momentum as electron spin‐
based quantum bit (qubit) candidates due to their synthetic tunability and long achievable …
based quantum bit (qubit) candidates due to their synthetic tunability and long achievable …
Chemical control of spin–lattice relaxation to discover a room temperature molecular qubit
MJ Amdur, KR Mullin, MJ Waters, D Puggioni… - Chemical …, 2022 - pubs.rsc.org
The second quantum revolution harnesses exquisite quantum control for a slate of diverse
applications including sensing, communication, and computation. Of the many candidates …
applications including sensing, communication, and computation. Of the many candidates …
Metal–ligand covalency enables room temperature molecular qubit candidates
MS Fataftah, MD Krzyaniak, B Vlaisavljevich… - Chemical …, 2019 - pubs.rsc.org
Harnessing synthetic chemistry to design electronic spin-based qubits, the smallest unit of a
quantum information system, enables us to probe fundamental questions regarding spin …
quantum information system, enables us to probe fundamental questions regarding spin …
Probing vibrational symmetry effects and nuclear spin economy principles in molecular spin qubits
The selection of molecular spin qubits with a long coherence time, T m, is a central task for
implementing molecule-based quantum technologies. Even if a sufficiently long T m can be …
implementing molecule-based quantum technologies. Even if a sufficiently long T m can be …
Decoherence in molecular electron spin qubits: Insights from quantum many-body simulations
Quantum states are described by wave functions whose phases cannot be directly
measured but which play a vital role in quantum effects such as interference and …
measured but which play a vital role in quantum effects such as interference and …
Effect of Coordination Geometry on Magnetic Properties in a Series of Cobalt (II) Complexes and Structural Transformation in Mother Liquor
The three Co (II) complexes [Co (bbp) 2][Co (NCS) 4]· 4DMF (1),[Co (bbp)(NCS) 2 (DMF)]·
2DMF (2), and [Co (bbp)(NCS) 2](3) have been synthesized and characterized by single …
2DMF (2), and [Co (bbp)(NCS) 2](3) have been synthesized and characterized by single …
Magnetic and relaxation properties of vanadium (iv) complexes: an integrated 1 H relaxometric, EPR and computational study
V Lagostina, F Carniato, D Esteban-Gómez… - Inorganic Chemistry …, 2023 - pubs.rsc.org
We report a detailed study of the magnetic and relaxation properties of a series of
oxovanadium (IV) complexes comprising the aqua ion [VO (H2O) 5] 2+ and [VO (ox) 2] …
oxovanadium (IV) complexes comprising the aqua ion [VO (H2O) 5] 2+ and [VO (ox) 2] …
Nuclear-spin-pattern control of electron-spin dynamics in a series of V (IV) complexes
Achieving control of phase memory relaxation times (Tm) in metal ions is an important goal
of molecular spintronics. Herein we provide the first evidence that nuclear-spin patterning in …
of molecular spintronics. Herein we provide the first evidence that nuclear-spin patterning in …
Understanding covalent versus spin–orbit coupling contributions to temperature-dependent electron spin relaxation in cupric and vanadyl phthalocyanines
Recent interest in transition-metal complexes as potential quantum bits (qubits) has
reinvigorated the investigation of fundamental contributions to electron spin relaxation in …
reinvigorated the investigation of fundamental contributions to electron spin relaxation in …
VdW Mediated Strong Magnetic Exchange Interactions in Chains of Hydrogen-Free Sublimable Molecular Qubits
Sulfur-rich molecular complexes of dithiolene-like ligands are appealing candidates as
molecular spin qubits because spin coherence properties are enhanced in hydrogen-free …
molecular spin qubits because spin coherence properties are enhanced in hydrogen-free …