Promises and challenges of next-generation “beyond Li-ion” batteries for electric vehicles and grid decarbonization

Y Tian, G Zeng, A Rutt, T Shi, H Kim, J Wang… - Chemical …, 2020 - ACS Publications
The tremendous improvement in performance and cost of lithium-ion batteries (LIBs) have
made them the technology of choice for electrical energy storage. While established battery …

Oxide cathodes: functions, instabilities, self healing, and degradation mitigations

Y Dong, J Li - Chemical Reviews, 2022 - ACS Publications
Recent progress in high-energy-density oxide cathodes for lithium-ion batteries has pushed
the limits of lithium usage and accessible redox couples. It often invokes hybrid anion-and …

Cation-disordered rocksalt-type high-entropy cathodes for Li-ion batteries

Z Lun, B Ouyang, DH Kwon, Y Ha, EE Foley… - Nature materials, 2021 - nature.com
Abstract High-entropy (HE) ceramics, by analogy with HE metallic alloys, are an emerging
class of solid solutions composed of a large number of species. These materials offer the …

Li-rich cathodes for rechargeable Li-based batteries: reaction mechanisms and advanced characterization techniques

W Zuo, M Luo, X Liu, J Wu, H Liu, J Li… - Energy & …, 2020 - pubs.rsc.org
Due to their high specific capacities beyond 250 mA hg− 1, lithium-rich oxides have been
considered as promising cathodes for the next generation power batteries, bridging the …

Cation-disordered rocksalt transition metal oxides and oxyfluorides for high energy lithium-ion cathodes

RJ Clément, Z Lun, G Ceder - Energy & Environmental Science, 2020 - pubs.rsc.org
For lithium-ion rechargeable batteries to meet society's ever-growing demands in electrical
energy storage, eg for the electrification of transportation, for portable electronics and for grid …

Multi-anionic and-cationic compounds: new high entropy materials for advanced Li-ion batteries

Q Wang, A Sarkar, D Wang, L Velasco… - Energy & …, 2019 - pubs.rsc.org
In the present work, a new class of high entropy materials for energy storage applications is
introduced. Multi-anionic and-cationic compounds are prepared by facile mechanochemistry …

Al‐doping driven suppression of capacity and voltage fadings in 4d‐element containing Li‐ion‐battery cathode materials: Machine learning and density functional …

M Ha, A Hajibabaei, DY Kim, AN Singh… - Advanced Energy …, 2022 - Wiley Online Library
The anion redox reaction in high‐energy‐density cathode materials such as Li‐excess
layered oxides suffers from voltage/capacity fadings due to irreversible structural instability …

Electrochemical ion insertion from the atomic to the device scale

A Sood, AD Poletayev, DA Cogswell… - Nature Reviews …, 2021 - nature.com
Electrochemical ion insertion involves coupled ion–electron transfer reactions, transport of
guest species and redox of the host. The hosts are typically anisotropic solids with 2D …

Design principles for zero-strain Li-ion cathodes

X Zhao, Y Tian, Z Lun, Z Cai, T Chen, B Ouyang… - Joule, 2022 - cell.com
The cycling of cathode materials for Li-ion batteries is often accompanied by a change in
volume, posing a challenge to the integrity of cathode particles and electrolyte/cathode …

Fundamentals of ion‐exchange synthesis and its implications in layered oxide cathodes: recent advances and perspective

Y Luo, Q Pan, H Wei, Y Huang, L Tang… - Advanced Energy …, 2023 - Wiley Online Library
Layered oxide cathodes such as Ni‐rich ternary and Li‐rich layered cathode materials have
been widely used for lithium‐ion batteries owing to their excellent Li+ transport properties …