Insights into low thermal conductivity in inorganic materials for thermoelectrics

T Ghosh, M Dutta, D Sarkar… - Journal of the American …, 2022 - ACS Publications
Efficient manipulation of thermal conductivity and fundamental understanding of the
microscopic mechanisms of phonon scattering in crystalline solids are crucial to achieve …

Cu 2 Se-Based liquid-like thermoelectric materials: looking back and stepping forward

Z Zhang, K Zhao, TR Wei, P Qiu, L Chen… - Energy & Environmental …, 2020 - pubs.rsc.org
High-performance liquid-like thermoelectrics have attracted global renewed attention since
the paradigm of 'phonon-liquid electron-crystal'was proposed in 2012. As one of the most …

Unified theory of thermal transport in crystals and glasses

M Simoncelli, N Marzari, F Mauri - Nature Physics, 2019 - nature.com
Crystals and glasses exhibit fundamentally different heat conduction mechanisms: the
periodicity of crystals allows for the excitation of propagating vibrational waves that carry …

Extremely low thermal conductivity and high electrical conductivity of sustainable carbonceramic electrospun nonwoven materials

X Liao, J Denk, T Tran, N Miyajima, L Benker… - Science …, 2023 - science.org
Materials with an extremely low thermal and high electrical conductivity that are easy to
process, foldable, and nonflammable are required for sustainable applications, notably in …

Wigner formulation of thermal transport in solids

M Simoncelli, N Marzari, F Mauri - Physical Review X, 2022 - APS
Two different heat-transport mechanisms are discussed in solids. In crystals, heat carriers
propagate and scatter particlelike as described by Peierls's formulation of the Boltzmann …

Isotropic Conduction Network and Defect Chemistry in Mg3+δ Sb2 -Based Layered Zintl Compounds with High Thermoelectric Performance.

H Tamaki, HK Sato, T Kanno - Advanced Materials (Deerfield Beach …, 2016 - europepmc.org
Thermoelectric performance in the layered Zintl phase n-type Mg 3+ δ (Sb, Bi) 2 is reported.
Insertion of the excess Mg into the compounds is crucial for realizing n-type carrier transport …

Orbitally driven giant phonon anharmonicity in SnSe

CW Li, J Hong, AF May, D Bansal, S Chi, T Hong… - Nature Physics, 2015 - nature.com
Understanding elementary excitations and their couplings in condensed matter systems is
critical for developing better energy-conversion devices. In thermoelectric materials, the heat …

On the tuning of electrical and thermal transport in thermoelectrics: an integrated theory–experiment perspective

J Yang, L Xi, W Qiu, L Wu, X Shi, L Chen… - NPJ Computational …, 2016 - nature.com
During the last two decades, we have witnessed great progress in research on
thermoelectrics. There are two primary focuses. One is the fundamental understanding of …

Single-atom vibrational spectroscopy in the scanning transmission electron microscope

FS Hage, G Radtke, DM Kepaptsoglou, M Lazzeri… - Science, 2020 - science.org
Single-atom impurities and other atomic-scale defects can notably alter the local vibrational
responses of solids and, ultimately, their macroscopic properties. Using high-resolution …

Anharmoncity and low thermal conductivity in thermoelectrics

C Chang, LD Zhao - Materials Today Physics, 2018 - Elsevier
The thermoelectric (TE) efficiency is evaluated by the material thermoelectric figure of merit
(ZT), which can be usually improved by enhancing the electrical transport properties and/or …