Challenges and recent advances in high capacity Li‐rich cathode materials for high energy density lithium‐ion batteries

W He, W Guo, H Wu, L Lin, Q Liu, X Han… - Advanced …, 2021 - Wiley Online Library
Li‐rich cathode materials have attracted increasing attention because of their high reversible
discharge capacity (> 250 mA hg− 1), which originates from transition metal (TM) ion redox …

[HTML][HTML] Pushing the limit of 3d transition metal-based layered oxides that use both cation and anion redox for energy storage

M Zhang, DA Kitchaev, Z Lebens-Higgins… - Nature Reviews …, 2022 - nature.com
Intercalation chemistry has dominated electrochemical energy storage for decades, and
storage capacity worldwide has now reached the terawatt-hour level. State-of-the-art …

Pushing lithium cobalt oxides to 4.7 V by lattice‐matched interfacial engineering

X Yang, C Wang, P Yan, T Jiao, J Hao… - Advanced Energy …, 2022 - Wiley Online Library
The utilization of high‐voltage LiCoO2 is imperative to break the bottleneck of the practical
energy density of lithium‐ion batteries. However, LiCoO2 suffers from severe structural and …

Improving the oxygen redox reversibility of Li-rich battery cathode materials via Coulombic repulsive interactions strategy

Q Li, D Ning, D Wong, K An, Y Tang, D Zhou… - Nature …, 2022 - nature.com
The oxygen redox reaction in lithium-rich layered oxide battery cathode materials generates
extra capacity at high cell voltages (ie,> 4.5 V). However, the irreversible oxygen release …

[HTML][HTML] First-cycle voltage hysteresis in Li-rich 3d cathodes associated with molecular O2 trapped in the bulk

RA House, GJ Rees, MA Pérez-Osorio, JJ Marie… - Nature Energy, 2020 - nature.com
Li-rich cathode materials are potential candidates for next-generation Li-ion batteries.
However, they exhibit a large voltage hysteresis on the first charge/discharge cycle, which …

[PDF][PDF] Decoupling the roles of Ni and Co in anionic redox activity of Li-rich NMC cathodes

B Li, Z Zhuo, L Zhang, A Iadecola, X Gao, J Guo… - Nature Materials, 2023 - nature.com
Abstract Li [Li x Ni y Mn z Co1− x− y− z] O2 (lithium-rich NMCs) are benchmark cathode
materials receiving considerable attention due to the abnormally high capacities resulting …

Li-rich cathodes for rechargeable Li-based batteries: reaction mechanisms and advanced characterization techniques

W Zuo, M Luo, X Liu, J Wu, H Liu, J Li… - Energy & …, 2020 - pubs.rsc.org
Due to their high specific capacities beyond 250 mA hg− 1, lithium-rich oxides have been
considered as promising cathodes for the next generation power batteries, bridging the …

Toward emerging two-dimensional nickel-based materials for electrochemical energy storage: Progress and perspectives

W Xu, X Zhao, F Zhan, Q He, H Wang, J Chen… - Energy Storage …, 2022 - Elsevier
Abstract Two-dimensional (2D) Ni-based materials have attracted considerable attention
due to their distinctive properties, including high electro-activity, large specific surface areas …

Recent breakthroughs and perspectives of high-energy layered oxide cathode materials for lithium ion batteries

J Liu, J Wang, Y Ni, K Zhang, F Cheng, J Chen - Materials Today, 2021 - Elsevier
Ni-rich layered oxides (NRLOs) and Li-rich layered oxides (LRLOs) have been considered
as promising next-generation cathode materials for lithium ion batteries (LIBs) due to their …

[HTML][HTML] Voltage decay and redox asymmetry mitigation by reversible cation migration in lithium-rich layered oxide electrodes

D Eum, B Kim, SJ Kim, H Park, J Wu, SP Cho, G Yoon… - Nature Materials, 2020 - nature.com
Despite the high energy density of lithium-rich layered-oxide electrodes, their real-world
implementation in batteries is hindered by the substantial voltage decay on cycling. This …