Sustainable production and degradation of plastics using microbes

SY Choi, Y Lee, HE Yu, IJ Cho, M Kang, SY Lee - Nature Microbiology, 2023 - nature.com
Plastics are indispensable in everyday life and industry, but the environmental impact of
plastic waste on ecosystems and human health is a huge concern. Microbial biotechnology …

Biocatalytic amide bond formation

M Lubberink, W Finnigan, SL Flitsch - Green Chemistry, 2023 - pubs.rsc.org
Amide bonds occur in over half of target compounds in medicinal chemistry patents, making
amide bond formation the most commonly performed reaction in the pharmaceutical …

Streamlining the synthesis of amides using Nickel-based nanocatalysts

J Gao, R Ma, F Poovan, L Zhang, H Atia… - Nature …, 2023 - nature.com
The synthesis of amides is a key technology for the preparation of fine and bulk chemicals in
industry, as well as the manufacture of a plethora of daily life products. Furthermore, it …

High-Loading Single-Atom Ru Catalysts Anchored on N-Doped Graphdiyne/γ-Graphyne Quantum Dots for Selective Hydrodehalogenation and Hydrodearomatization

C Zhang, Y Li, Y Xie, Z Yu, X Wan, X Wang, J He… - ACS …, 2023 - ACS Publications
Selective hydrodehalogenation and hydrodearomatization of toxic chlorophenols into value-
added chemicals represents a grand challenge for their efficient reutilization. For this …

Enzymatic Oxy‐and Amino‐Functionalization in Biocatalytic Cascade Synthesis: Recent Advances and Future Perspectives

E Grandi, F Feyza Özgen, S Schmidt… - Angewandte …, 2023 - Wiley Online Library
Biocatalytic cascades are a powerful tool for building complex molecules containing oxygen
and nitrogen functionalities. Moreover, the combination of multiple enzymes in one pot offers …

One‐step biocatalytic synthesis of sustainable surfactants by selective amide bond formation

M Lubberink, W Finnigan, C Schnepel… - Angewandte Chemie …, 2022 - Wiley Online Library
Abstract N‐alkanoyl‐N‐methylglucamides (MEGAs) are non‐toxic surfactants widely used
as commercial ingredients, but more sustainable syntheses towards these compounds are …

Recent advances in the sustainable production of α, ω-C6 bifunctional compounds enabled by chemo-/biocatalysts

Q Li, Z Zhang, J Zhao, A Li - Green Chemistry, 2022 - pubs.rsc.org
α, ω-C6 bifunctional compounds play fundamental roles in the synthesis of a variety of value-
added products including polymers, adhesives, pharmaceuticals, perfumes and so on. So …

Multi-enzymatic cascade reactions with Escherichia coli-based modules for synthesizing various bioplastic monomers from fatty acid methyl esters

HW Yoo, H Jung, S Sarak, YC Kim, BG Park, BG Kim… - Green …, 2022 - pubs.rsc.org
Multi-enzymatic cascade reaction systems were designed to generate biopolymer
monomers using Escherichia coli-based cell modules, capable of carrying out one-pot …

Recent developments in oxidative biocatalytic cascades

WWL See, JPS Choo, DY Jung, L Zhi - Current Opinion in Green and …, 2022 - Elsevier
Biocatalytic cascades that involve enzymatic oxidation as one or more key steps are
powerful tools to access valuable chemicals with various functionalizations starting from …

Biocatalytic carboxylate reduction–recent advances and new enzymes

M Winkler, JG Ling - ChemCatChem, 2022 - Wiley Online Library
Carboxylate reductases (CARs) are valuable catalysts for the selective one‐step reduction
of carboxylic acids to their corresponding aldehydes. In recent years, numerous new CARs …