Fracture and adhesion of soft materials: a review

C Creton, M Ciccotti - Reports on Progress in Physics, 2016 - iopscience.iop.org
Soft materials are materials with a low shear modulus relative to their bulk modulus and
where elastic restoring forces are mainly of entropic origin. A sparse population of strong …

Recent advances on designs and applications of hydrogel adhesives

X Liu, H Yu, L Wang, Z Huang, F Haq… - Advanced Materials …, 2022 - Wiley Online Library
In virtue of extracellular features, hydrogels have been used in various areas such as tissue
repair, artificial skins, and biological electronics, etc. Intact contact of tough hydrogels to …

50th anniversary perspective: Networks and gels: Soft but dynamic and tough

C Creton - Macromolecules, 2017 - ACS Publications
Soft polymer networks have seen an explosion of recent developments motivated by new
high tech applications in the biomedical field or in engineering. We present a candid and …

Hydrogen-bond association-mediated dynamics and viscoelastic properties of tough supramolecular hydrogels

C Du, XN Zhang, TL Sun, M Du, Q Zheng… - Macromolecules, 2021 - ACS Publications
Forming robust associative interactions has been an effective strategy for the design of
tough hydrogels. However, the role of associative interactions in the dynamics of hydrogels …

Self-healing behaviors of tough polyampholyte hydrogels

AB Ihsan, TL Sun, T Kurokawa, SN Karobi… - …, 2016 - ACS Publications
Recently, polyampolytes have been discovered to form hydrogels that possess high
toughness, full resilience, and self-healing between two cut surfaces. The self-healing of this …

Molecular structure of self-healing polyampholyte hydrogels analyzed from tensile behaviors

TL Sun, F Luo, T Kurokawa, SN Karobi, T Nakajima… - Soft matter, 2015 - pubs.rsc.org
Recently, charge balanced polyampholytes (PA) have been found to form tough and self-
healing hydrogels. This class of physical hydrogels have a very high equilibrated polymer …

Strong and tough polyion-complex hydrogels from oppositely charged polyelectrolytes: A comparative study with polyampholyte hydrogels

F Luo, TL Sun, T Nakajima, DR King… - …, 2016 - ACS Publications
Oppositely charged homopolyelectrolytes were found to form strong, tough, and self-healing
polyion-complex (PIC) hydrogels, similar to polyampholytes (PA) which have opposite …

Supramolecular soft adhesive materials

J Courtois, I Baroudi, N Nouvel… - Advanced Functional …, 2010 - Wiley Online Library
The rheological and adhesive properties of bis‐urea functionalized low‐molecular‐weight
polyisobutylenes (PIBUT) are investigated. The polymers, which can interact through …

Waterborne Polyurethane− Acrylic hybrid nanoparticles by Miniemulsion polymerization: applications in pressure-sensitive adhesives

A Lopez, E Degrandi-Contraires, E Canetta, C Creton… - Langmuir, 2011 - ACS Publications
Waterborne polyurethane− acrylic hybrid nanoparticles for application as pressure-sensitive
adhesives (PSAs) were prepared by one-step miniemulsion polymerization. The addition of …

Effect of hydrophobic side group on structural heterogeneities and mechanical performance of gelatin-based hydrogen-bonded hydrogel

HJ Zhang, X Wang, Y Yang, TL Sun, A Zhang… - …, 2022 - ACS Publications
Hydrogen bonds stabilized by hydrophobic side groups have been widely applied to realize
high toughness of hydrogels. Herein, we studied the effect of the content of the hydrophobic …