Molecular qubits based on photogenerated spin-correlated radical pairs for quantum sensing
T Mani - Chemical Physics Reviews, 2022 - pubs.aip.org
Photogenerated spin-correlated radical pairs (SCRPs) in electron donor–bridge–acceptor
(D–B–A) molecules can act as molecular qubits and inherently spin qubit pairs. SCRPs can …
(D–B–A) molecules can act as molecular qubits and inherently spin qubit pairs. SCRPs can …
Spontaneous exciton dissociation enables spin state interconversion in delayed fluorescence organic semiconductors
Engineering a low singlet-triplet energy gap (ΔE ST) is necessary for efficient reverse
intersystem crossing (rISC) in delayed fluorescence (DF) organic semiconductors but results …
intersystem crossing (rISC) in delayed fluorescence (DF) organic semiconductors but results …
How quantum is radical pair magnetoreception?
Currently the most likely mechanism of the magnetic compass sense in migratory songbirds
relies on the coherent spin dynamics of pairs of photochemically formed radicals in the …
relies on the coherent spin dynamics of pairs of photochemically formed radicals in the …
Spin-selective electron transfer reactions of radical pairs: Beyond the Haberkorn master equation
Radical pair recombination reactions are normally described using a quantum mechanical
master equation for the electronic and nuclear spin density operator. The electron spin state …
master equation for the electronic and nuclear spin density operator. The electron spin state …
[HTML][HTML] Radical pair intersystem crossing: Quantum dynamics or incoherent kinetics?
TP Fay, DE Manolopoulos - The Journal of chemical physics, 2019 - pubs.aip.org
Magnetic field effects on radical pair reactions arise due to the interplay of coherent electron
spin dynamics and spin relaxation effects, a rigorous treatment of which requires the solution …
spin dynamics and spin relaxation effects, a rigorous treatment of which requires the solution …
Pulse sequences for manipulating the spin states of molecular radical-pair-based electron spin qubit systems for quantum information applications
GJ Pazera, MD Krzyaniak… - The Journal of Chemical …, 2023 - pubs.aip.org
Molecular qubits are an emerging platform in quantum information science due to the
unmatched structural control that chemical design and synthesis provide compared to other …
unmatched structural control that chemical design and synthesis provide compared to other …
Magnetic control of recombination fluorescence and tunability by modulation of radical pair energies in rigid donor–bridge–acceptor systems
JT Buck, T Mani - Journal of the American Chemical Society, 2020 - ACS Publications
Magnetic control of molecular emission holds the promise of developing new magneto-
optical technologies. Spin dynamics of radical pairs can serve as a basis of control of …
optical technologies. Spin dynamics of radical pairs can serve as a basis of control of …
Photoinduced intercomponent processes in selectively addressable bichromophoric dyads made of linearly arranged Ru (II) terpyridine and expanded pyridinium …
Three new linearly arranged bichromophoric systems 1–3 have been prepared, and their
photophysical properties have been studied, taking also advantage of femtosecond pump …
photophysical properties have been studied, taking also advantage of femtosecond pump …
Electron spin relaxation in radical pairs: Beyond the Redfield approximation
Relaxation processes can have a large effect on the spin selective electron transfer
reactions of radical pairs. These processes are often treated using phenomenological …
reactions of radical pairs. These processes are often treated using phenomenological …
Spin Dynamics of Radical Pairs Using the Stochastic Schrödinger Equation in MolSpin
The chemical reactivity of radical pairs is strongly influenced by the interactions of electronic
and nuclear spins. A detailed understanding of these effects requires a quantum description …
and nuclear spins. A detailed understanding of these effects requires a quantum description …