Ring-polymer molecular dynamics: Quantum effects in chemical dynamics from classical trajectories in an extended phase space

S Habershon, DE Manolopoulos… - Annual review of …, 2013 - annualreviews.org
This article reviews the ring-polymer molecular dynamics model for condensed-phase
quantum dynamics. This model, which involves classical evolution in an extended ring …

[HTML][HTML] Neural network potentials for chemistry: concepts, applications and prospects

S Käser, LI Vazquez-Salazar, M Meuwly, K Töpfer - Digital Discovery, 2023 - pubs.rsc.org
Artificial Neural Networks (NN) are already heavily involved in methods and applications for
frequent tasks in the field of computational chemistry such as representation of potential …

[HTML][HTML] Nuclear quantum effects on zeolite proton hopping kinetics explored with machine learning potentials and path integral molecular dynamics

M Bocus, R Goeminne, A Lamaire… - Nature …, 2023 - nature.com
Proton hopping is a key reactive process within zeolite catalysis. However, the accurate
determination of its kinetics poses major challenges both for theoreticians and …

How to remove the spurious resonances from ring polymer molecular dynamics

M Rossi, M Ceriotti, DE Manolopoulos - The Journal of chemical …, 2014 - pubs.aip.org
Two of the most successful methods that are presently available for simulating the quantum
dynamics of condensed phase systems are centroid molecular dynamics (CMD) and ring …

Ring-polymer molecular dynamics rate-theory in the deep-tunneling regime: Connection with semiclassical instanton theory

JO Richardson, SC Althorpe - The Journal of chemical physics, 2009 - pubs.aip.org
We demonstrate that the ring-polymer molecular dynamics (RPMD) method is equivalent to
an automated and approximate implementation of the “Im F” version of semiclassical …

How quantum is the resonance behavior in vibrational polariton chemistry?

MR Fiechter, JE Runeson, JE Lawrence… - The Journal of …, 2023 - ACS Publications
Recent experiments in polariton chemistry have demonstrated that reaction rates can be
modified by vibrational strong coupling to an optical cavity mode. Importantly, this …

Determining the three-phase coexistence line in methane hydrates using computer simulations

MM Conde, C Vega - The Journal of chemical physics, 2010 - pubs.aip.org
Molecular dynamics simulations have been performed to estimate the three-phase (solid
hydrate-liquid water-gaseous methane) coexistence line for the water-methane binary …

On the applicability of centroid and ring polymer path integral molecular dynamics for vibrational spectroscopy

A Witt, SD Ivanov, M Shiga, H Forbert… - The Journal of chemical …, 2009 - pubs.aip.org
Centroid molecular dynamics (CMD) and ring polymer molecular dynamics (RPMD) are two
conceptually distinct extensions of path integral molecular dynamics that are able to …

Chemical reaction rate coefficients from ring polymer molecular dynamics: Theory and practical applications

YV Suleimanov, FJ Aoiz, H Guo - The Journal of Physical …, 2016 - ACS Publications
This Feature Article presents an overview of the current status of ring polymer molecular
dynamics (RPMD) rate theory. We first analyze the RPMD approach and its connection to …

Bimolecular reaction rates from ring polymer molecular dynamics: Application to H+ CH4→ H2+ CH3

YV Suleimanov, R Collepardo-Guevara… - The Journal of …, 2011 - pubs.aip.org
In a recent paper, we have developed an efficient implementation of the ring polymer
molecular dynamics (RPMD) method for calculating bimolecular chemical reaction rates in …