Time-resolved ARPES studies of quantum materials

F Boschini, M Zonno, A Damascelli - Reviews of Modern Physics, 2024 - APS
Angle-resolved photoemission spectroscopy (ARPES), with its exceptional sensitivity to both
the binding energy and the momentum of valence electrons in solids, provides unparalleled …

Advancing time-and angle-resolved photoemission spectroscopy: The role of ultrafast laser development

MX Na, AK Mills, DJ Jones - Physics Reports, 2023 - Elsevier
In the last decade, there has been a proliferation of laser sources for time-and angle-
resolved photoemission spectroscopy (TR-ARPES), building on the proven capability of this …

Spin-polarized spatially indirect excitons in a topological insulator

R Mori, S Ciocys, K Takasan, P Ai, K Currier… - Nature, 2023 - nature.com
The exciton, a bound state of an electron and a hole, is a fundamental quasiparticle induced
by coherent light–matter interactions in semiconductors. When the electrons and holes are …

Helicity dependent photocurrent in electrically gated (Bi1−xSbx)2Te3 thin films

Y Pan, QZ Wang, AL Yeats, T Pillsbury… - Nature …, 2017 - nature.com
Circularly polarized photons are known to generate a directional helicity-dependent
photocurrent in three-dimensional topological insulators at room temperature. Surprisingly …

Narrowband, Angle-Tunable, Helicity-Dependent Terahertz Emission from Nanowires of the Topological Dirac Semimetal Cd3As2

JL Boland, DA Damry, CQ Xia, P Schönherr… - ACS …, 2023 - ACS Publications
All-optical control of terahertz pulses is essential for the development of optoelectronic
devices for next-generation quantum technologies. Despite substantial research in THz …

Band-resolved imaging of photocurrent in a topological insulator

H Soifer, A Gauthier, AF Kemper, CR Rotundu… - Physical Review Letters, 2019 - APS
We study the microscopic origins of photocurrent generation in the topological insulator Bi 2
Se 3 via time-and angle-resolved photoemission spectroscopy. We image the unoccupied …

Electron– versus Spin–Phonon Coupling Governs the Temperature-Dependent Carrier Dynamics in the Topological Insulator Bi2Te3

H Lu, R Long, WH Fang - Journal of the American Chemical …, 2023 - ACS Publications
Ultrafast charge and spin dynamics have immense effects on the applications of topological
insulators (TIs). By performing spin-adiabatic nonadiabatic molecular dynamics simulations …

A first-principles time-dependent density functional theory framework for spin and time-resolved angular-resolved photoelectron spectroscopy in periodic systems

U De Giovannini, H Hübener… - Journal of chemical theory …, 2017 - ACS Publications
We present a novel theoretical approach to simulate spin, time, and angular-resolved
photoelectron spectroscopy (ARPES) from first-principles that is applicable to surfaces, thin …

Terahertz probe of nonequilibrium carrier dynamics and ultrafast photocurrents in the topological insulator Sb2Te3

S Ruan, X Lin, H Chen, B Song, Y Dai, X Yan… - Applied Physics …, 2021 - pubs.aip.org
In this study, we report the ultrafast excitation and dynamics of the carrier and photocurrent
in a 3D typical topological insulator Sb 2 Te 3. We utilize time-resolved optical pump-THz …

Time-and angle-resolved photoemission studies of quantum materials

F Boschini, M Zonno, A Damascelli - arXiv preprint arXiv:2309.03935, 2023 - arxiv.org
Angle-resolved photoemission spectroscopy (ARPES)--with its exceptional sensitivity to both
the binding energy and momentum of valence electrons in solids--provides unparalleled …