Optimizing the electrocatalytic selectivity of carbon dioxide reduction reaction by regulating the electronic structure of single‐atom M‐N‐C materials

T Tang, Z Wang, J Guan - Advanced Functional Materials, 2022 - Wiley Online Library
Electrochemical carbon dioxide reduction reaction (CO2RR) is an efficient strategy to relieve
global environmental and energy issues by converting excess CO2 from the atmosphere to …

Tuning the coordination environment of carbon‐based single‐atom catalysts via doping with multiple heteroatoms and their applications in electrocatalysis

Z Qi, Y Zhou, R Guan, Y Fu, JB Baek - Advanced Materials, 2023 - Wiley Online Library
Carbon‐based single‐atom catalysts (SACs) are considered to be a perfect platform for
studying the structure–activity relationship of different reactions due to the adjustability of …

Unveiling the Proton‐Feeding Effect in Sulfur‐Doped Fe−N−C Single‐Atom Catalyst for Enhanced CO2 Electroreduction

S Chen, X Li, CW Kao, T Luo, K Chen… - Angewandte Chemie …, 2022 - Wiley Online Library
Heteroatom‐doping in metal‐nitrogen‐carbon single‐atom catalysts (SACs) is considered a
powerful strategy to promote the electrocatalytic CO2 reduction reaction (CO2RR), but the …

[HTML][HTML] Attenuating metal-substrate conjugation in atomically dispersed nickel catalysts for electroreduction of CO2 to CO

Q Wang, K Liu, K Hu, C Cai, H Li, H Li, M Herran… - Nature …, 2022 - nature.com
Atomically dispersed transition metals on carbon-based aromatic substrates are an
emerging class of electrocatalysts for the electroreduction of CO2. However, electron …

[HTML][HTML] Acidic CO2-to-HCOOH electrolysis with industrial-level current on phase engineered tin sulfide

H Shen, H Jin, H Li, H Wang, J Duan, Y Jiao… - Nature …, 2023 - nature.com
Acidic CO2-to-HCOOH electrolysis represents a sustainable route for value-added CO2
transformations. However, competing hydrogen evolution reaction (HER) in acid remains a …

Design of Co‐Cu Diatomic Site Catalysts for High‐efficiency Synergistic CO2 Electroreduction at Industrial‐level Current Density

J Yi, X Gao, H Zhou, W Chen… - Angewandte Chemie …, 2022 - Wiley Online Library
Single atom catalysts (SACs) have been widely studied in the field of CO2 electroreduction,
but industrial‐level current density and near‐unity product selectivity are still difficult to …

High-Efficiency N2 Electroreduction Enabled by Se-Vacancy-Rich WSe2–x in Water-in-Salt Electrolytes

P Shen, X Li, Y Luo, Y Guo, X Zhao, K Chu - ACS nano, 2022 - ACS Publications
Electrocatalytic nitrogen reduction reaction (NRR) is a promising approach for renewable
NH3 production, while developing the NRR electrocatalysis systems with both high activity …

[HTML][HTML] Accelerated water activation and stabilized metal-organic framework via constructing triangular active-regions for ampere-level current density hydrogen …

F Cheng, X Peng, L Hu, B Yang, Z Li, CL Dong… - Nature …, 2022 - nature.com
Two-dimensional metal-organic frameworks (MOFs) have been explored as effective
electrocatalysts for hydrogen evolution reaction (HER). However, the sluggish water …

[PDF][PDF] Electronic structure regulation of single-site MNC electrocatalysts for carbon dioxide reduction

T Tang, Z Wang, J Guan - Acta Phys.–Chim. Sin, 2022 - whxb.pku.edu.cn
The current global population and economy depends on fossil fuel consumption; however,
the uncontrolled exploitation of fossil fuels has caused a series of energy crises and …

Asymmetric Coordination Induces Electron Localization at Ca Sites for Robust CO2 Electroreduction to CO

Q Wang, M Dai, H Li, YR Lu, TS Chan, C Ma… - Advanced …, 2023 - Wiley Online Library
Main group single atom catalysts (SACs) are promising for CO2 electroreduction to CO by
virtue of their ability in preventing the hydrogen evolution reaction and CO poisoning …