Siloxane coordination revisited: Si− O bond character, reactivity and magnificent molecular shapes

F Dankert, C von Hänisch - European Journal of Inorganic …, 2021 - Wiley Online Library
Siloxanes have evolved into a multi‐million dollar business due to their manifold of
commercial and industrial applications. As siloxanes have high hydrophobicity, low basicity …

Recent advances in organo-lanthanides and actinides mediated hydroaminations

H Liu, S Saha, MS Eisen - Coordination Chemistry Reviews, 2023 - Elsevier
Hydroamination, an atom-economic one-step reaction that refers to the addition of an NH
unit into CC/CX multiple bonds, provides an ideally efficient methodology to construct C–N …

Reduction vs. addition: the reaction of an aluminyl anion with 1, 3, 5, 7‐cyclooctatetraene

RJ Schwamm, MD Anker, M Lein… - Angewandte Chemie …, 2019 - Wiley Online Library
The potassium aluminyl complex K [Al (NONAr)](NON= NONAr=[O (SiMe2NAr) 2] 2−, Ar= 2,
6‐iPr2C6H3) reacts with 1, 3, 5, 7‐cyclooctatetraene (COT) to give K [Al (NONAr)(COT)]. The …

Self-assembly of Keggin-type U (VI)-containing tungstophosphates with a sandwich structure: an efficient catalyst for the synthesis of sulfonyl pyrazoles

GP Yang, XL Zhang, YF Liu, DD Zhang, K Li… - Inorganic Chemistry …, 2021 - pubs.rsc.org
The reaction of UO2 (OAc) 2 and Na9 [A-PW9O34] in solution with different pH values leads
to the formation of two Keggin-type sandwich polyoxometalates, namely Na11H (H2O) 31 …

Zinc Catalyzed Hydroelementation (HE; E= B, C, N, and O) of Carbodiimides: Intermediates Isolation and Mechanistic Insights

RK Sahoo, AG Patro, N Sarkar, S Nembenna - Organometallics, 2023 - ACS Publications
The conjugated bis-guanidinate (CBG) supported zinc hydride,[{LZnH} 2; L={(ArHN)(ArN)-
C═ N–C═(NAr)(NHAr); Ar= 2, 6-Et2-C6H3}](1)(pre)-catalyzed addition of E–H (E= B, C, N …

Recent developments in highly basic N-heterocyclic iminato ligands in actinide chemistry

S Revathi, P Raja, S Saha, MS Eisen… - Chemical …, 2021 - pubs.rsc.org
In the last decade, major conceptual advances in the chemistry of actinide molecules and
materials have been made to demonstrate their distinct reactivity profiles as compared to …

The role of 5f-orbital participation in unexpected inversion of the σ-bond metathesis reactivity trend of triamidoamine thorium (IV) and uranium (IV) alkyls

BM Gardner, PA Cleaves, CE Kefalidis, J Fang… - Chemical …, 2014 - pubs.rsc.org
We report on the role of 5f-orbital participation in the unexpected inversion of the σ-bond
metathesis reactivity trend of triamidoamine thorium (IV) and uranium (IV) alkyls. Reaction of …

Actinide‐Mediated Catalytic Addition of E H Bonds (E= N, P, S) to Carbodiimides, Isocyanates, and Isothiocyanates

ISR Karmel, M Tamm, MS Eisen - … Chemie International Edition, 2015 - Wiley Online Library
Unprecedented catalytic reactivity of actinide coordination complexes toward
heterocumulenes, such as carbodiimides, isocyanates, and isothiocyanates is reported. The …

Mono (imidazolin-2-iminato) actinide complexes: synthesis and application in the catalytic dimerization of aldehydes

ISR Karmel, N Fridman, M Tamm… - Journal of the American …, 2014 - ACS Publications
The synthesis of the mono (imidazolin-2-iminato) actinide (IV) complexes [(ImRN) An (N
{SiMe3) 2} 3](3–8) was accomplished by the protonolysis reaction between the respective …

Effect of Na(I)-H2O clusters on self-assembly of sandwich-type U(VI)-containing silicotungstates and the efficient catalytic activity for the synthesis of substituted phenylsulfonyl-1 …

K Li, XL Lin, K Zeng, XF Gao, W Cen, YF Liu, GP Yang - Tungsten, 2022 - Springer
In this study, a sandwich-type uranium (VI)-containing silicotungstate KNa 11 H 2 (H 2 O) 30
[Na (UO 2)(SiW 9 O 34)] 2· 8H 2 O (1) with new three-dimensional (3D) structure was …