Hydrogenase enzymes and their synthetic models: the role of metal hydrides

D Schilter, JM Camara, MT Huynh… - Chemical …, 2016 - ACS Publications
Hydrogenase enzymes efficiently process H2 and protons at organometallic FeFe, NiFe, or
Fe active sites. Synthetic modeling of the many H2ase states has provided insight into …

Hydrogenases

W Lubitz, H Ogata, O Rudiger, E Reijerse - Chemical reviews, 2014 - ACS Publications
The reaction takes place at a specialized metal center that dramatically increases the acidity
of H2 and leads to a heterolytic splitting of the molecule which is strongly accelerated by the …

Hydrogen evolution catalyzed by cobaloximes

JL Dempsey, BS Brunschwig, JR Winkler… - Accounts of chemical …, 2009 - ACS Publications
Natural photosynthesis uses sunlight to drive the conversion of energy-poor molecules
(H2O, CO2) to energy-rich ones (O2,(CH2O) n). Scientists are working hard to develop …

Structural and functional analogues of the active sites of the [Fe]-,[NiFe]-, and [FeFe]-hydrogenases

C Tard, CJ Pickett - Chemical reviews, 2009 - ACS Publications
This article sets out to review the chemistry relating to the synthesis of structural and
functional analogues of the three classes of hydrogenases. This chemistry has grown …

Hydrogen-oxidizing bacteria and their applications in resource recovery and pollutant removal

L Lin, H Huang, X Zhang, L Dong, Y Chen - Science of The Total …, 2022 - Elsevier
Hydrogen oxidizing bacteria (HOB), a type of chemoautotroph, are a group of bacteria from
different genera that share the ability to oxidize H 2 and fix CO 2 to provide energy and …

DFT study on structure, electronic properties, and reactivity of cis-isomers of [(NC5H4-S)2Fe(CO)2]

CA Mebi - Journal of Chemical Sciences, 2011 - Springer
Three cis-isomers of [(NC 5 H 4-S) 2 Fe (CO) 2], models for the active site of [Fe]
hydrogenase, have been examined by computational method at DFT B3LYP/6–311+ G (d …

Hydrogenase enzymes: recent structural studies and active site models

DM Heinekey - Journal of Organometallic Chemistry, 2009 - Elsevier
Hydrogenase enzymes: Recent structural studies and active site models - ScienceDirect
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Hydrogenases and oxygen

MT Stiebritz, M Reiher - Chemical science, 2012 - pubs.rsc.org
Hydrogenases represent a heterogeneous group of enzymes consisting of three
evolutionary unrelated classes, ie [NiFe],[FeFe] and [Fe] hydrogenases. They allow the uni …

Spectroscopic Investigations of [FeFe] Hydrogenase Maturated with [57Fe2(adt)(CN)2(CO)4]2–

R Gilbert-Wilson, JF Siebel… - Journal of the …, 2015 - ACS Publications
The preparation and spectroscopic characterization of a CO-inhibited [FeFe] hydrogenase
with a selectively 57Fe-labeled binuclear subsite is described. The precursor [57Fe2 …

A personal account on 25 years of scientific literature on [FeFe]-hydrogenase

JW Sidabras, ST Stripp - JBIC Journal of Biological Inorganic Chemistry, 2023 - Springer
Abstract [FeFe]-hydrogenases are gas-processing metalloenzymes that catalyze H2
oxidation and proton reduction (H2 release) in microorganisms. Their high turnover …