Skeletal editing through direct nitrogen deletion of secondary amines

SH Kennedy, BD Dherange, KJ Berger, MD Levin - Nature, 2021 - nature.com
Synthetic chemistry aims to build up molecular complexity from simple feedstocks. However,
the ability to exert precise changes that manipulate the connectivity of the molecular …

Anomeric amides—structure, properties and reactivity

SA Glover - Tetrahedron, 1998 - Elsevier
Amides, geminally substituted with two heteroatoms at nitrogen, can support anomeric
effects in much the same way as their carbon analogues such as acetals and aminals. To …

Pd(II)-Catalyzed Cross-Coupling of sp3 C−H Bonds with sp2 and sp3 Boronic Acids Using Air as the Oxidant

DH Wang, M Wasa, R Giri, JQ Yu - Journal of the American …, 2008 - ACS Publications
O-Methyl hydroxamic acids, readily available from carboxylic acids, are found to be
extremely reactive for β-C− H activation by Pd (OAc) 2. This reactivity is exploited to develop …

[图书][B] The Chemistry of Hydroxylamines, Oximes and Hydroxamic Acids, Volume 1

Z Rappoport, JF Liebman - 2008 - books.google.com
Page 1 Patai Series: The Chemistry of Functional Groups Series Editor: Zvi Rappoport Volume
Editors: Zvi Rappoport & Joel F. Liebman The Chemistry of Hyd roxylamines, Oximes and …

Ambient and aerobic carbon–carbon bond cleavage toward α-ketoester synthesis by transition-metal-free photocatalysis

Q Yu, Y Zhang, JP Wan - Green Chemistry, 2019 - pubs.rsc.org
The α-oxoesterification of the CC double bond in readily available enaminones enabling
efficient synthesis of α-ketoesters is developed. The reactions showing general tolerance to …

Ligand-enabled β-C–H arylation of α-amino acids using a simple and practical auxiliary

G Chen, T Shigenari, P Jain, Z Zhang… - Journal of the …, 2015 - ACS Publications
Pd-catalyzed β-C–H functionalizations of carboxylic acid derivatives using an auxiliary as a
directing group have been extensively explored in the past decade. In comparison to the …

[HTML][HTML] Heteroatom substitution at amide nitrogen—resonance reduction and HERON reactions of anomeric amides

SA Glover, AA Rosser - Molecules, 2018 - mdpi.com
This review describes how resonance in amides is greatly affected upon substitution at
nitrogen by two electronegative atoms. Nitrogen becomes strongly pyramidal and resonance …

Direct ester condensation from a 1: 1 mixture of carboxylic acids and alcohols catalyzed by hafnium (IV) or zirconium (IV) salts

K Ishihara, M Nakayama, S Ohara, H Yamamoto - Tetrahedron, 2002 - Elsevier
To promote atom efficiency in synthesis and to avoid the generation of environmental waste,
the use of stoichiometric amounts of condensing reagents or excess substrates should be …

Transition-Metal-Assisted Radical/Radical Cross-Coupling: A New Strategy to the Oxidative C(sp3)–H/N–H Cross-Coupling

L Zhou, S Tang, X Qi, C Lin, K Liu, C Liu, Y Lan… - Organic …, 2014 - ACS Publications
A transition-metal-assisted oxidative C (sp3)-H/N–H cross-coupling reaction of N-
alkoxyamides with aliphatic hydrocarbons is described. During the reaction, nitrogen …

Palladium-Catalyzed Alkoxylation of N-Methoxybenzamides via Direct sp2 C−H Bond Activation

GW Wang, TT Yuan - The Journal of Organic Chemistry, 2010 - ACS Publications
The palladium-catalyzed ortho-alkoxylation of N-methoxybenzamides has been
demonstrated. With the CONHOMe group as a directing group, the aromatic C− H bond can …