Click chemistry strategies for the accelerated synthesis of functional macromolecules

Z Geng, JJ Shin, Y Xi, CJ Hawker - Journal of Polymer Science, 2021 - Wiley Online Library
Click chemistry is one of the most powerful strategies for constructing polymeric soft
materials with precise control over architecture and functionality. In this review, we provide a …

Synthetic strategies, properties, and applications of unsaturated main-chain metallopolymers prepared by olefin metathesis polymerization

Y Sha, H Jia, Z Shen, Z Luo - Polymer Reviews, 2021 - Taylor & Francis
Main-chain metallopolymers are synthesized by olefin metathesis polymerizations. These
polymers are mainly produced through acyclic diene metathesis (ADMET) polymerization …

SPAAC iClick: progress towards a bioorthogonal reaction in-corporating metal ions

YH Shen, AM Esper, I Ghiviriga, KA Abboud… - Dalton …, 2021 - pubs.rsc.org
Combining strain-promoted azide–alkyne cycloaddition (SPAAC) and inorganic click (iClick)
reactivity provides access to metal 1, 2, 3-triazolates. Experimental and computational …

Understanding the solubilization of Ca acetylide with a new computational model for ionic pairs

MV Polynski, MD Sapova, VP Ananikov - Chemical Science, 2020 - pubs.rsc.org
The unique reactivity of the acetylenic unit in DMSO gives rise to ubiquitous synthetic
methods. We theoretically consider CaC2 solubility and protolysis in DMSO and formulate a …

Trapping of Terminal Platinapolyynes by Copper (I) Catalyzed Click Cycloadditions; Probes of Labile Intermediates in Syntheses of Complexes with Extended sp …

H Amini, N Weisbach, S Gauthier… - … A European Journal, 2021 - Wiley Online Library
The silylated hexatriynyl complex trans‐(C6F5)(p‐tol3P) 2Pt (C≡ C) 3SiEt3 (PtC6TES) is
converted in situ to PtC6H (wet n‐Bu4N+ F−, THF) and cross coupled with the diyne H (C≡ …

Electrospray Mass Spectrometry to Study Combinatorial iClick Reactions and Multiplexed Kinetics of [Ru(N3)(N∧N)(terpy)]PF6 with Alkynes of Different Steric and …

T Zach, F Geyer, B Kiendl, J Mößeler… - Inorganic …, 2023 - ACS Publications
In a combinatorial approach, a family of ruthenium (II) azido complexes [Ru (N3)(N∧
N)(terpy)] PF6 with terpy= 2, 2′: 6′, 2 ″-terpyridine and N∧ N as a bidentate chelator …

N^ N^ C platinum (II) complexes based on phenyl-pyridin-2-ylpyrimidine ligands: synthesis, electrochemical and photophysical properties

M Hruzd, S Gauthier, J Boixel, S Kahlal, N Le Poul… - Dyes and …, 2021 - Elsevier
A series of luminescent chloro-and alkynyl-platinum (II) complexes containing various
tridentate cyclometalated ligands derived from phenyl-pyridin-2-ylpyrimidine and alkynyl …

C^ N^ N Coordination Accelerates the iClick Reaction of Square-Planar Palladium (II) and Platinum (II) Azido Complexes with Electron-Poor Alkynes and Enables …

K Peng, D Moreth, U Schatzschneider - Organometallics, 2021 - ACS Publications
Organometal azido complexes with a cyclometalating C^ N^ N coligand of the general
formula [M (N3)(phbpy)] with M= Pd (II) or Pt (II) and Hphbpy= 6-phenyl-2, 2′-bipyridine …

iClick synthesis of network metallopolymers

YH Shen, I Ghiviriga, KA Abboud, KS Schanze… - Dalton …, 2022 - pubs.rsc.org
Described is an approach to preparing the first iClick network metallopolymers with porous
properties. Treating digoldazido complex 2-AuN3 with trigoldacetylide 3-AuPPh3 or 3 …

The iClick Reaction of a BODIPY Platinum(II) Azido Complex with Electron-Poor Alkynes Provides Triazolate Complexes with Good 1O2 Sensitization Efficiency

K Peng, R Einsele, P Irmler, RF Winter… - …, 2020 - ACS Publications
trans-[Pt (bodipy)(N3)(PEt3) 2](bodipy= 4, 4-difluoro-4-bora-3 a, 4 a-diaza-s-indacen-8-yl;
Et= ethyl) reacts with dimethyl acetylenedicarboxylate (DMAD) or F3C–C≡ C–COOEt in a …