Thermal energy transport in oxide nuclear fuel

DH Hurley, A El-Azab, MS Bryan, MWD Cooper… - Chemical …, 2021 - ACS Publications
To efficiently capture the energy of the nuclear bond, advanced nuclear reactor concepts
seek solid fuels that must withstand unprecedented temperature and radiation extremes. In …

Multipolar interactions in -electron systems: The paradigm of actinide dioxides

P Santini, S Carretta, G Amoretti, R Caciuffo… - Reviews of Modern …, 2009 - APS
This article reviews the physics of multipolar interactions and multipolar order in f-electron
systems, using the actinide dioxides as a paradigm. In the past few years, these apparently …

calculations of the ground state and metastable states of uranium dioxide

B Dorado, B Amadon, M Freyss, M Bertolus - Physical Review B—Condensed …, 2009 - APS
We report a study of the ground state and metastable states of uranium dioxide using ab
initio DFT+ U calculations. We highlight that in order to avoid metastable states and …

Stability of oxygen point defects in by first-principles calculations: Occupation matrix control and Jahn-Teller distortion

B Dorado, G Jomard, M Freyss, M Bertolus - Physical Review B—Condensed …, 2010 - APS
Point-defect formation energies in uranium dioxide UO 2 are still a matter of debate due to
the significant discrepancies between the various studies published in the literature. These …

Hybrid Density-Functional Theory and the Insulating Gap of

KN Kudin, GE Scuseria, RL Martin - Physical Review Letters, 2002 - APS
We report the first calculations carried out with a periodic boundary condition code capable
of examining hybrid density-functional theory (DFT) for f-element solids. We apply it to the …

U and Xe transport in UO: Density functional theory calculations

DA Andersson, BP Uberuaga, PV Nerikar, C Unal… - Physical Review B …, 2011 - APS
The detrimental effects of the fission gas Xe on the performance of oxide nuclear fuels are
well known. However, less well known are the mechanisms that govern fission gas …

Anisotropic thermal conductivity in uranium dioxide

K Gofryk, S Du, CR Stanek, JC Lashley, XY Liu… - Nature …, 2014 - nature.com
The thermal conductivity of uranium dioxide has been studied for over half a century, as
uranium dioxide is the fuel used in a majority of operating nuclear reactors and thermal …

Triple- Octupolar Ordering in

JA Paixão, C Detlefs, MJ Longfield, R Caciuffo… - Physical review …, 2002 - APS
We report the results of resonant x-ray scattering experiments performed at the Np M 4, 5
edges in N p O 2. Below T 0= 25 K, the development of long-range order of Np electric …

Magnetic structure and electric-field gradients of uranium dioxide: An ab initio study

R Laskowski, GKH Madsen, P Blaha, K Schwarz - Physical Review B, 2004 - APS
The magnetic structure of uranium dioxide has been investigated using linear augmented
plane wave ab initio calculations, taking into account spin-orbit coupling, strong Coulomb …

First-principles calculation and experimental study of oxygen diffusion in uranium dioxide

B Dorado, P Garcia, G Carlot, C Davoisne… - Physical Review B …, 2011 - APS
This work provides an illustration that density functional theory (DFT)+ U calculations may
quantitatively describe transport phenomena in uranium dioxide. Oxygen diffusion …