Over the past fifteen years or so, the study of f-element single-ion magnets (f-SIMs) has gone
from being a sub-discipline of molecular magnetism to an established field of research in its …

Over recent decades, much effort has been made to lengthen spin relaxation/decoherence
times of single-molecule magnets and molecular qubits by following different chemical …

Quantum coherence is detected in the 4f single-ion magnet (SIM) Yb (trensal), by isotope
selective pulsed EPR spectroscopy on an oriented single crystal. At X-band, the spin–lattice …

To design molecular spin qubits and nanomagnets operating at high temperatures, there is
an urgent need to understand the relationship between vibrations and spin relaxation …

Conspectus Longstanding and important applications make use of the chemical and
physical properties of both rare earth metals and polyoxometalates of early transition metals …

We study the quantum spin dynamics of nearly isotropic Gd 3+ ions entrapped in
polyoxometalate molecules and diluted in crystals of a diamagnetic Y 3+ derivative. The full …

Realizing atomic-level spatial control over qubits, the fundamental units of both quantum
information processing systems and quantum sensors, constitutes a crucial cross-field …

Enabling the rational synthesis of molecular candidates for quantum information processing
requires design principles that minimize electron spin decoherence. Here we report a …

Single-ion magnets (SIMs) are mononuclear molecular complexes exhibiting slow relaxation
of magnetization. They are currently attracting a lot of interest because of potential …

We report a vanadium complex in a nuclear-spin free ligand field that displays two key
properties for an ideal candidate qubit system: long coherence times that persist at high …