Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Enrichment of reactants and intermediates for electrocatalytic CO 2 reduction

PP Yang, MR Gao - Chemical Society Reviews, 2023 - pubs.rsc.org
The electrocatalytic carbon dioxide reduction reaction (CO2RR) presents a sustainable
route to convert renewable electricity to value-added fuels and feedstocks in the form of …

Electrochemical C–N coupling of CO 2 and nitrogenous small molecules for the electrosynthesis of organonitrogen compounds

X Peng, L Zeng, D Wang, Z Liu, Y Li, Z Li… - Chemical Society …, 2023 - pubs.rsc.org
Electrochemical C–N coupling reactions based on abundant small molecules (such as CO2
and N2) have attracted increasing attention as a new “green synthetic strategy” for the …

Gas diffusion electrodes and membranes for CO2 reduction electrolysers

EW Lees, BAW Mowbray, FGL Parlane… - Nature Reviews …, 2022 - nature.com
The CO2 reduction reaction (CO2RR) is a potential means of using renewable electricity to
synthesize commodity chemicals and fuels. The CO2RR can be performed at industrially …

Close to 90% Single-Pass Conversion Efficiency for CO2 Electroreduction in an Acid-Fed Membrane Electrode Assembly

B Pan, J Fan, J Zhang, Y Luo, C Shen, C Wang… - ACS Energy …, 2022 - ACS Publications
The formation of (bi) carbonates is a pressing issue for CO2 electroreduction in neutral or
alkaline solutions. It adversely causes low single-pass conversion efficiency as a result of …

Membrane Electrode Assembly for Electrocatalytic CO2 Reduction: Principle and Application

Z Zhang, X Huang, Z Chen, J Zhu… - Angewandte …, 2023 - Wiley Online Library
Electrocatalytic CO2 reduction reaction (CO2RR) in membrane electrode assembly (MEA)
systems is a promising technology. Gaseous CO2 can be directly transported to the cathode …

Bipolar membrane electrolyzers enable high single-pass CO2 electroreduction to multicarbon products

K Xie, RK Miao, A Ozden, S Liu, Z Chen… - Nature …, 2022 - nature.com
In alkaline and neutral MEA CO2 electrolyzers, CO2 rapidly converts to (bi) carbonate,
imposing a significant energy penalty arising from separating CO2 from the anode gas …

Zero-Gap Electrochemical CO2 Reduction Cells: Challenges and Operational Strategies for Prevention of Salt Precipitation

M Sassenburg, M Kelly, S Subramanian… - ACS Energy …, 2022 - ACS Publications
Salt precipitation is a problem in electrochemical CO2 reduction electrolyzers that limits their
long-term durability and industrial applicability by reducing the active area, causing flooding …

Carbon-efficient carbon dioxide electrolysers

A Ozden, FP García de Arquer, JE Huang, J Wicks… - Nature …, 2022 - nature.com
The electroreduction of CO2 (CO2R) is the conversion of CO2 to renewable fuels and
feedstocks, a promising technology that could support the transition from fossil to renewable …

Highly selective and productive reduction of carbon dioxide to multicarbon products via in situ CO management using segmented tandem electrodes

T Zhang, JC Bui, Z Li, AT Bell, AZ Weber, J Wu - Nature Catalysis, 2022 - nature.com
Electrochemical CO2 reduction provides a promising route to the sustainable generation of
valuable chemicals and fuels. Tandem catalysts enable sequential CO2-to-CO and CO-to …