Two-dimensional (2D) optical spectroscopy utilizing multiple ultrafast coherent laser pulses
in the infrared or UV-vis frequency range has been used to study protein structure and …

In this review the basis, recent developments and applications of coherent anti-Stokes
Raman scattering (CARS) in the fields of spectroscopy and microscopy are dialed with. The …

We have demonstrated that fifth-order stimulated Raman spectra of the intermolecular
modes in CS 2 are dominated by cascading third-order processes. Previous studies have …

Coherent multidimensional vibrational spectroscopy (CMDVS) is an emerging field that
offers new oportunities to probe specifically intramolecular and intermolecular interactions in …

The vibrations of condensed phase molecules are a topic of great interest because they
provide a spectroscopic window into molecular structures, dynamics, and their surrounding …

We present a classical theoretical treatment of a two-dimensional Raman spectroscopy
based on the initiation of vibrational coherence with an impulsive Raman pump and …

The two-dimensional infrared-infrared-visible (IIV) sum frequency generation (SFG) is
theoretically considered. IIV-SFG is a two-dimensional extension of the infrared-visible SFG …

The cascading polarization contributing to the femtosecond fifth-and seventh-order coherent
Raman scattering processes is obtained in terms of the third-and fifth-order Raman …

A variety of two-dimensional 2D vibrational spectroscopies have shown to be useful
methods in studying vibrational couplings and dynamics of polyatomic molecules, 1–20 eg …

Phenomena associated with the breakdown of inversion symmetry in the HD molecule are
reviewed and discussed. A distinction is made between three kinds of physical effects …