Soft materials by design: unconventional polymer networks give extreme properties

X Zhao, X Chen, H Yuk, S Lin, X Liu… - Chemical Reviews, 2021 - ACS Publications
Hydrogels are polymer networks infiltrated with water. Many biological hydrogels in animal
bodies such as muscles, heart valves, cartilages, and tendons possess extreme mechanical …

Hydrogels for flexible electronics

Y Zhang, Y Tan, J Lao, H Gao, J Yu - ACS nano, 2023 - ACS Publications
Hydrogels have emerged as promising materials for flexible electronics due to their unique
properties, such as high water content, softness, and biocompatibility. In this perspective, we …

Fracture, fatigue, and friction of polymers in which entanglements greatly outnumber cross-links

J Kim, G Zhang, M Shi, Z Suo - Science, 2021 - science.org
In gels and elastomers, the role of entanglements on deformation has been studied, but their
effects on fracture, fatigue, and friction are less well understood. In this study, we …

Phase-locked constructing dynamic supramolecular ionic conductive elastomers with superior toughness, autonomous self-healing and recyclability

J Chen, Y Gao, L Shi, W Yu, Z Sun, Y Zhou… - Nature …, 2022 - nature.com
Stretchable ionic conductors are considerable to be the most attractive candidate for next-
generation flexible ionotronic devices. Nevertheless, high ionic conductivity, excellent …

Strong, tough, rapid-recovery, and fatigue-resistant hydrogels made of picot peptide fibres

B Xue, Z Bashir, Y Guo, W Yu, W Sun, Y Li… - Nature …, 2023 - nature.com
Hydrogels are promising soft materials as tissue engineering scaffolds, stretchable sensors,
and soft robotics. Yet, it remains challenging to develop synthetic hydrogels with mechanical …

Coordinatively stiffen and toughen hydrogels with adaptable crystal‐domain cross‐linking

L Xu, Y Qiao, D Qiu - Advanced Materials, 2023 - Wiley Online Library
Conventional hydrogels usually suffer from the inherent conflict between stiffness and
toughness, severely hampering their applications as load‐bearing materials. Herein, an …

Entanglement in Smart Hydrogels: Fast Response Time, Anti‐Freezing and Anti‐Drying

Y Feng, S Wang, Y Li, W Ma, G Zhang… - Advanced Functional …, 2023 - Wiley Online Library
The common techniques to improve hydrogel's mechanical properties include increasing
crosslinking density and forming crosslinked double‐network hydrogel, which may cause …

Design principles for strong and tough hydrogels

X Li, JP Gong - Nature Reviews Materials, 2024 - nature.com
Hydrogels are crosslinked polymer networks swollen with water. Owing to their soft and
water-containing nature, hydrogels are promising materials for applications in many fields …

Creep-free polyelectrolyte elastomer for drift-free iontronic sensing

Y He, Y Cheng, C Yang, CF Guo - Nature Materials, 2024 - nature.com
Artificial pressure sensors often use soft materials to achieve skin-like softness, but the
viscoelastic creep of soft materials and the ion leakage, specifically for ionic conductors …

Insertion of Urea Moieties for One‐Component Strong yet Tough, Self‐Healing Polyurea Protective Materials

Z Zhang, L Qian, G Huang, C Chen… - Advanced Functional …, 2024 - Wiley Online Library
Polyurea has gained increasing attention in civil engineering, flexible electronics, and other
emerging fields. However, owing to the rapid polymerization, tailoring their mechanical …