Single-atom logic for heterocycle editing

J Jurczyk, J Woo, SF Kim, BD Dherange, R Sarpong… - Nature …, 2022 - nature.com
Medicinal chemistry continues to be impacted by new synthetic methods. Particularly sought
after, especially at the drug discovery stage, is the ability to enact the desired chemical …

Kinetics, spectroscopy, and computational chemistry of arylnitrenes

NP Gritsan, MS Platz - Chemical reviews, 2006 - ACS Publications
Arylnitrenes are very reactive and short-lived intermediates commonly generated by
decomposition of aryl azides. Although other arylnitrene precursors are known1 and their …

Tandem C/N-difunctionalization of nitroarenes: reductive amination and annulation by a ring expansion/contraction sequence

G Li, MN Lavagnino, SZ Ali, S Hu… - Journal of the …, 2022 - ACS Publications
A synthetic method for the reductive transformation of nitroarenes into ortho-aminated and-
annulated products is reported. The method operates via the exhaustive deoxygenation of …

A Photochemical Strategy for ortho‐Aminophenol Synthesis via Dearomative‐Rearomative Coupling Between Aryl Azides and Alcohols

B Li, A Ruffoni, D Leonori - Angewandte Chemie International …, 2023 - Wiley Online Library
Abstract ortho‐Aminophenols are aromatic derivatives featuring vicinal N‐and O‐based
functionalities commonly found in the structures of many high‐value materials. These …

[图书][B] CRC Handbook of Organic Photochemistry and Photobiology, Volumes 1 & 2

WM Horspool, F Lenci - 2003 - taylorfrancis.com
The second edition of this best-selling handbook is bigger, more comprehensive, and now
completely current. In addition to thorough updates to the discussions featured in the first …

An Improved PIII/PV═O-Catalyzed Reductive C–N Coupling of Nitroaromatics and Boronic Acids by Mechanistic Differentiation of Rate- and Product-Determining …

G Li, TV Nykaza, JC Cooper, A Ramirez… - Journal of the …, 2020 - ACS Publications
Experimental, spectroscopic, and computational studies are reported that provide an
evidence-based mechanistic description of an intermolecular reductive C–N coupling of …

Recent progress on reductive coupling of nitroarenes by using organosilanes as convenient reductants

Y Gao, S Yang, Y Huo, XQ Hu - Advanced Synthesis & …, 2020 - Wiley Online Library
Nitroarenes are stable, low‐cost, and readily available starting materials. The directly utilize
nitroarenes in synthetically valuable C− N bond formation is of great significance, because …

Photochemical reactions in the synthesis of protein–drug conjugates

JP Holland, M Gut, S Klingler, R Fay… - … –A European Journal, 2020 - Wiley Online Library
The ability to modify biologically active molecules such as antibodies with drug molecules,
fluorophores or radionuclides is crucial in drug discovery and target identification. Classic …

Study of the Chemistry of ortho- and para-Biphenylnitrenes by Laser Flash Photolysis and Time-Resolved IR Experiments and by B3LYP and CASPT2 Calculations

ML Tsao, N Gritsan, TR James, MS Platz… - Journal of the …, 2003 - ACS Publications
The photochemistry of ortho-biphenyl azide (1a) has been studied by laser flash photolysis
(LFP), with UV− vis and IR detection of the transient intermediates formed. LFP (266 nm) of …

Charting the Chemical and Mechanistic Scope of Light-Triggered Protein Ligation

DF Earley, A Guillou, S Klingler, R Fay, M Gut… - JACS Au, 2022 - ACS Publications
The creation of discrete, covalent bonds between a protein and a functional molecule like a
drug, fluorophore, or radiolabeled complex is essential for making state-of-the-art tools that …