Two-dimensional electronic spectroscopy

E Fresch, FVA Camargo, Q Shen, CC Bellora… - Nature Reviews …, 2023 - nature.com
Two-dimensional electronic spectroscopy (2DES) is a popular technique that can track
ultrafast coherent and incoherent processes in real time. Since its development in the late …

Photosynthetic light harvesting: excitons and coherence

F Fassioli, R Dinshaw, PC Arpin… - Journal of The Royal …, 2014 - royalsocietypublishing.org
Photosynthesis begins with light harvesting, where specialized pigment–protein complexes
transform sunlight into electronic excitations delivered to reaction centres to initiate charge …

Roadmap on quantum light spectroscopy

S Mukamel, M Freyberger, W Schleich… - Journal of physics B …, 2020 - iopscience.iop.org
Conventional spectroscopy uses classical light to detect matter properties through the
variation of its response with frequencies or time delays. Quantum light opens up new …

Coherence in Chemistry: Foundations and Frontiers

JD Schultz, JL Yuly, EA Arsenault, K Parker… - Chemical …, 2024 - ACS Publications
Coherence refers to correlations in waves. Because matter has a wave-particle nature, it is
unsurprising that coherence has deep connections with the most contemporary issues in …

Nonlinear optical signals and spectroscopy with quantum light

KE Dorfman, F Schlawin, S Mukamel - Reviews of Modern Physics, 2016 - APS
Conventional nonlinear spectroscopy uses classical light to detect matter properties through
the variation of its response with frequencies or time delays. Quantum light opens up new …

Energy transfer pathways in semiconducting carbon nanotubes revealed using two-dimensional white-light spectroscopy

RD Mehlenbacher, TJ McDonough, M Grechko… - Nature …, 2015 - nature.com
Thin film networks of highly purified semiconducting carbon nanotubes (CNTs) are being
explored for energy harvesting and optoelectronic devices because of their exceptional …

Probing homogeneous line broadening in CdSe nanocrystals using multidimensional electronic spectroscopy

TA Gellen, J Lem, DB Turner - Nano Letters, 2017 - ACS Publications
The finite spectral line width of an ensemble of CdSe nanocrystals arises from size and
shape inhomogeneity and the single-nanocrystal spectrum itself. This line width directly …

Steady-state analysis of light-harvesting energy transfer driven by incoherent light: From dimers to networks

PY Yang, J Cao - The journal of physical chemistry letters, 2020 - ACS Publications
The question of how quantum coherence facilitates energy transfer has been intensively
debated in the scientific community. Since natural and artificial light-harvesting units operate …

First evidence of purely extreme-ultraviolet four-wave mixing

L Foglia, F Capotondi, R Mincigrucci, D Naumenko… - Physical Review Letters, 2018 - APS
The extension of nonlinear optical techniques to the extreme-ultraviolet (EUV), soft and hard
x-ray regime represents one of the open challenges of modern science since it would …

Coherent multi-dimensional spectroscopy: Experimental considerations, direct comparisons and new capabilities

JO Tollerud, JA Davis - Progress in Quantum Electronics, 2017 - Elsevier
Abstract Optical Coherent Multidimensional Spectroscopy (CMDS) has been developed to
probe the electronic states of a diverse range of complex systems. The great advantage of …