Time-domain observation of interlayer exciton formation and thermalization in a MoSe2/WSe2 heterostructure

VR Policht, H Mittenzwey, O Dogadov, M Katzer… - Nature …, 2023 - nature.com
Vertical heterostructures of transition metal dichalcogenides (TMDs) host interlayer excitons
with electrons and holes residing in different layers. With respect to their intralayer …

Strong Coupling of Coherent Phonons to Excitons in Semiconducting Monolayer MoTe2

CJ Sayers, A Genco, C Trovatello, SD Conte… - Nano Letters, 2023 - ACS Publications
The coupling of the electron system to lattice vibrations and their time-dependent control and
detection provide unique insight into the nonequilibrium physics of semiconductors. Here …

Exciton-phonon scattering: Competition between the bosonic and fermionic nature of bound electron-hole pairs

M Katzer, M Selig, L Sigl, M Troue, J Figueiredo… - Physical Review B, 2023 - APS
The question of macroscopic occupation and the spontaneous emergence of coherence for
exciton ensembles has gained renewed attention due to the rise of van der Waals …

A roadmap to decipher ultrafast photophysics in two-dimensional nanomaterials

P Schiettecatte, Z Hens, P Geiregat - The Journal of chemical physics, 2023 - pubs.aip.org
Atomically thin two-dimensional (2D) semiconductors are extensively investigated for
optoelectronic applications that require strong light–matter interactions. In view of such …

Auger‐Assisted Secondary Hot Carrier Transfer in a Type I MoS2/PtSe2 Heterostructure

J Yang, S Gong, X Zhang, J Liu, W Luo… - Advanced Functional …, 2024 - Wiley Online Library
Charge transfer is vital in determining the optoelectronic properties of atomically thin
materials, yet remains elusive in type I heterostructures. Here, distinct two‐step charge …

Ultrafast Optical Control of Exciton Diffusion in WSe2/Graphene Heterostructures Revealed by Heterodyne Transient Grating Spectroscopy

L Rieland, J Wagner, R Bernhardt, T Wang… - Nano Letters, 2024 - ACS Publications
Using heterodyne transient grating spectroscopy, we observe a significant enhancement of
exciton diffusion in a monolayer WSe2 stacked on graphene. The diffusion dynamics can be …

Detection of a Coherent Excitonic State in the Layered Semiconductor BiI3

V Gosetti, J Cervantes-Villanueva, D Sangalli… - ACS …, 2024 - ACS Publications
The measurement and manipulation of the coherent dynamics of excitonic states constitute a
forefront research challenge in semiconductor optics and quantum-coherence-based …

Trion formation resolves observed peak shifts in the optical spectra of transition-metal dichalcogenides

T Sayer, YR Farah, R Austin, J Sambur… - Nano Letters, 2023 - ACS Publications
Monolayer transition-metal dichalcogenides (ML-TMDs) have the potential to unlock novel
photonic and chemical technologies if their optoelectronic properties can be understood and …

Excitonic effect drives ultrafast transition in two-dimensional transition metal dichalcogenides

SW Zheng, HY Wang, H Wang… - The Journal of Physical …, 2023 - ACS Publications
Two-dimensional (2D) transition metal dichalcogenides (TMDCs) are ideal platforms for
exploring excitonic physics because of the tightly bound excitons. In this work, we observed …

Chirality-Dependent Dynamic Evolution for Trions in Monolayer WS2

B Xiang, R Wang, Y Chen, Y Wang, T Qin, M Zhang… - Nano Letters, 2024 - ACS Publications
Monolayer transition metal dichalcogenides exhibit valley-dependent excitonic characters
with a large binding energy, acting as the building block for future optoelectronic …