Semiconductor quantum dots: Technological progress and future challenges

FP García de Arquer, DV Talapin, VI Klimov, Y Arakawa… - Science, 2021 - science.org
BACKGROUND Semiconductor materials feature optical and electronic properties that can
be engineered through their composition and crystal structure. The use of semiconductors …

Oriented attachment: from natural crystal growth to a materials engineering tool

BBV Salzmann, MM Van Der Sluijs… - Accounts of chemical …, 2021 - ACS Publications
Conspectus Intuitively, chemists see crystals grow atom-by-atom or molecule-by-molecule,
very much like a mason builds a wall, brick by brick. It is much more difficult to grasp that …

Colloidal synthesis path to 2D crystalline quantum dot superlattices

JC Ondry, JP Philbin, M Lostica, E Rabani… - ACS …, 2020 - ACS Publications
By combining colloidal nanocrystal synthesis, self-assembly, and solution phase epitaxial
growth techniques, we developed a general method for preparing single dot thick atomically …

PbI2 Passivation of Three Dimensional PbS Quantum Dot Superlattices Toward Optoelectronic Metamaterials

J Pinna, E Pili, R Mehrabi Koushki, DS Gavhane… - ACS …, 2024 - ACS Publications
Lead chalcogenide colloidal quantum dots are one of the most promising materials to
revolutionize the field of short-wavelength infrared optoelectronics due to their bandgap …

Neck barrier engineering in quantum dot dimer molecules via intraparticle ripening

J Cui, S Koley, YE Panfil, A Levi, Y Ossia… - Journal of the …, 2021 - ACS Publications
Coupled colloidal quantum dot (CQD) dimers represent a new class of artificial molecules
composed of fused core/shell semiconductor nanocrystals. The electronic coupling and …

Quantum dot acceptors in two-dimensional epitaxially fused PbSe quantum dot superlattices

V Notot, W Walravens, M Berthe, N Peric, A Addad… - ACS …, 2022 - ACS Publications
Oriented attachment of colloidal quantum dots allows the growth of two-dimensional crystals
by design, which could have striking electronic properties upon progress on manipulating …

In situ super-hindrance-triggered multilayer cracks for random lasing in π-functional nanopolymer films

D Lin, Y Li, H Zhang, S Zhang, Y Gao, T Zhai, S Hu… - Research, 2023 - spj.science.org
In situ self-assembly of semiconducting emitters into multilayer cracks is a significant
solution-processing method to fabricate organic high-Q lasers. However, it is still difficult to …

Mapping Defect Relaxation in Quantum Dot Solids upon In Situ Heating

MA Smeaton, I El Baggari, DM Balazs, T Hanrath… - ACS …, 2021 - ACS Publications
Epitaxially connected quantum dot solids have emerged as an interesting class of quantum
confined materials with the potential for highly tunable electronic structures. Realization of …

An artificial intelligence's interpretation of complex high-resolution in situ transmission electron microscopy data

X Wang, C Yan, JC Ondry, V Bodiwala, P Ercius… - Matter, 2024 - cell.com
Complicated nano-and atomic-scale processes with sub-angstrom spatial resolution and
millisecond time resolution visualized by in situ transmission electron microscopy (TEM) are …

Application of dislocation theory to minimize defects in artificial solids built with nanocrystal building blocks

JC Ondry, AP Alivisatos - Accounts of chemical research, 2021 - ACS Publications
Conspectus Oriented atomic attachment of colloidal inorganic nanocrystals represents a
powerful synthetic method for preparing complex inorganic superstructures. Examples …