Photons, Excitons, and Electrons in Covalent Organic Frameworks

D Blätte, F Ortmann, T Bein - Journal of the American Chemical …, 2024 - ACS Publications
Covalent organic frameworks (COFs) are created by the condensation of molecular building
blocks and nodes to form two-dimensional (2D) or three-dimensional (3D) crystalline …

The Molecular Nature of Redox-Conductive Metal–Organic Frameworks

J Li, S Ott - Accounts of Chemical Research, 2024 - ACS Publications
Conspectus Redox-conductive metal–organic frameworks (RC-MOFs) are a class of porous
materials that exhibit electrical conductivity through a chain of self-exchange reactions …

Electronic spin qubit candidates arrayed within layered two-dimensional polymers

AK Oanta, KA Collins, AM Evans… - Journal of the …, 2022 - ACS Publications
Molecular electronic spin qubits are promising candidates for quantum information science
applications because they can be reliably produced and engineered via chemical design …

Synthesis, hole doping, and electrical properties of a semiconducting azatriangulene-based covalent organic framework

DW Burke, RR Dasari, VK Sangwan… - Journal of the …, 2023 - ACS Publications
Two-dimensional covalent organic frameworks (2D COFs) containing heterotriangulenes
have been theoretically identified as semiconductors with tunable, Dirac-cone-like band …

Experimental manifestation of redox-conductivity in metal-organic frameworks and its implication for semiconductor/insulator switching

J Li, A Kumar, BA Johnson, S Ott - Nature Communications, 2023 - nature.com
Electric conductivity in metal-organic frameworks (MOFs) follows either a band-like or a
redox-hopping charge transport mechanism. While conductivity by the band-like mechanism …

π-Stacks of radical-anionic naphthalenediimides in a metal-organic framework

B Kim, J Lee, YP Chen, XQ Wu, J Kang, H Jeong… - Science …, 2022 - science.org
Radical-ionic metal-organic frameworks (MOFs) have unique optical, magnetic, and
electronic properties. These radical ions, forcibly formed by external stimulus-induced redox …

Backbone coplanarity manipulation via hydrogen bonding to boost the n-type performance of polymeric mixed conductors operating in aqueous electrolyte

J Chen, S Cong, L Wang, Y Wang, L Lan, C Chen… - Materials …, 2023 - pubs.rsc.org
The development of high-performance n-type semiconducting polymers remains a
significant challenge. Reported here is the construction of a coplanar backbone via …

Tailoring COFs: Transforming Nonconducting 2D Layered COF into a Conducting Quasi-3D Architecture via Interlayer Knitting with Polypyrrole

C Jain, R Kushwaha, D Rase, P Shekhar… - Journal of the …, 2023 - ACS Publications
Improving the electronic conductivity and the structural robustness of covalent organic
frameworks (COFs) is paramount. Here, we covalently cross-link a 2D COF with polypyrrole …

2D Conjugated polymer thin films for organic electronics: opportunities and challenges

G Fu, H Yang, W Zhao, P Samorì… - Advanced Materials, 2024 - Wiley Online Library
Abstract 2D conjugated polymers (2DCPs) possess extended in‐plane π‐conjugated lattice
and out‐of‐plane π–π stacking, which results in enhanced electronic performance and …

Synthesis of ruthenium-based metallo-covalent organic frameworks for efficient photocatalytic ring opening of α-ketoepoxides under visible light

M Wang, Z Li, Q Xiong, A Song, Y Lu, R Wang… - Journal of Catalysis, 2023 - Elsevier
Abstract Two-dimensional (2D) metallo-covalent organic frameworks (MCOFs) have been
regarded as an interesting new class of photoactive materials due to their superior thermal …