Stability Issues in Electrochemical CO2 Reduction: Recent Advances in Fundamental Understanding and Design Strategies

W Lai, Y Qiao, Y Wang, H Huang - Advanced Materials, 2023 - Wiley Online Library
Electrochemical CO2 reduction reaction (CO2RR) offers a promising approach to close the
anthropogenic carbon cycle and store intermittent renewable energy in fuels or chemicals …

Heterogeneous Molecular Catalysts of Metal Phthalocyanines for Electrochemical CO2 Reduction Reactions

Y Wu, Y Liang, H Wang - Accounts of Chemical Research, 2021 - ACS Publications
Conspectus Molecular catalysts, often deployed in homogeneous conditions, are favorable
systems for structure–reactivity correlation studies of electrochemical reactions because of …

Coverage-driven selectivity switch from ethylene to acetate in high-rate CO2/CO electrolysis

P Wei, D Gao, T Liu, H Li, J Sang, C Wang… - Nature …, 2023 - nature.com
Tuning catalyst microenvironments by electrolytes and organic modifications is effective in
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …

Electrocatalytic CO2-to-C2+ with Ampere-Level Current on Heteroatom-Engineered Copper via Tuning *CO Intermediate Coverage

M Zheng, P Wang, X Zhi, K Yang, Y Jiao… - Journal of the …, 2022 - ACS Publications
An ampere-level current density of CO2 electrolysis is critical to realize the industrial
production of multicarbon (C2+) fuels. However, under such a large current density, the poor …

Bioinspired and bioderived aqueous electrocatalysis

J Barrio, A Pedersen, S Favero, H Luo, M Wang… - Chemical …, 2022 - ACS Publications
The development of efficient and sustainable electrochemical systems able to provide clean-
energy fuels and chemicals is one of the main current challenges of materials science and …

Homogeneous Vacancies-Enhanced Orbital Hybridization for Selective and Efficient CO2-to-CO Electrocatalysis

Y Qin, G Zhan, C Tang, D Yang, X Wang, J Yang… - Nano Letters, 2023 - ACS Publications
Crafting vacancies offers an efficient route to upgrade the selectivity and productivity of
nanomaterials for CO2 electroreduction. However, defective nanoelectrocatalysts bear …

Hydrophobicity Graded Gas Diffusion Layer for Stable Electrochemical Reduction of CO2

L Li, J Chen, VSS Mosali, Y Liang… - Angewandte Chemie …, 2022 - Wiley Online Library
To mitigate flooding associated with the gas diffusion layer (GDL) during electroreduction of
CO2, we report a hydrophobicity‐graded hydrophobic GDL (HGGDL). Coating uniformly …

Superhydrophobicity-Enabled Efficient Electrocatalytic CO2 Reduction at a High Temperature

K Li, S Zou, J Zhang, Y Huang, L He, X Feng - ACS Catalysis, 2023 - ACS Publications
Enhancing the electrocatalytic CO2 reduction reaction (CO2RR) by a temperature increase
is very attractive, but lower CO2 solubility and the more intense competitive hydrogen …

CO2 Electrolyzers

CP O'Brien, RK Miao, A Shayesteh Zeraati… - Chemical …, 2024 - ACS Publications
CO2 electrolyzers have progressed rapidly in energy efficiency and catalyst selectivity
toward valuable chemical feedstocks and fuels, such as syngas, ethylene, ethanol, and …

Electrocatalytic CO2 Reduction to Ethylene: From Advanced Catalyst Design to Industrial Applications

T Lu, T Xu, S Zhu, J Li, J Wang, H Jin… - Advanced …, 2023 - Wiley Online Library
The value‐added chemicals, monoxide, methane, ethylene, ethanol, ethane, and so on, can
be efficiently generated through the electrochemical CO2 reduction reaction (eCO2RR) …