FAIR data enabling new horizons for materials research

M Scheffler, M Aeschlimann, M Albrecht, T Bereau… - Nature, 2022 - nature.com
The prosperity and lifestyle of our society are very much governed by achievements in
condensed matter physics, chemistry and materials science, because new products for …

Extending machine learning beyond interatomic potentials for predicting molecular properties

N Fedik, R Zubatyuk, M Kulichenko, N Lubbers… - Nature Reviews …, 2022 - nature.com
Abstract Machine learning (ML) is becoming a method of choice for modelling complex
chemical processes and materials. ML provides a surrogate model trained on a reference …

Artificial intelligence for science in quantum, atomistic, and continuum systems

X Zhang, L Wang, J Helwig, Y Luo, C Fu, Y Xie… - arXiv preprint arXiv …, 2023 - arxiv.org
Advances in artificial intelligence (AI) are fueling a new paradigm of discoveries in natural
sciences. Today, AI has started to advance natural sciences by improving, accelerating, and …

Machine‐Learning‐Assisted Determination of the Global Zero‐Temperature Phase Diagram of Materials

J Schmidt, N Hoffmann, HC Wang, P Borlido… - Advanced …, 2023 - Wiley Online Library
Crystal‐graph attention neural networks have emerged recently as remarkable tools for the
prediction of thermodynamic stability. The efficacy of their learning capabilities and their …

A perspective on sustainable computational chemistry software development and integration

R Di Felice, ML Mayes, RM Richard… - Journal of chemical …, 2023 - ACS Publications
The power of quantum chemistry to predict the ground and excited state properties of
complex chemical systems has driven the development of computational quantum chemistry …

SchNetPack 2.0: A neural network toolbox for atomistic machine learning

KT Schütt, SSP Hessmann, NWA Gebauer… - The Journal of …, 2023 - pubs.aip.org
SchNetPack is a versatile neural network toolbox that addresses both the requirements of
method development and the application of atomistic machine learning. Version 2.0 comes …

Operando modeling of zeolite-catalyzed reactions using first-principles molecular dynamics simulations

V Van Speybroeck, M Bocus, P Cnudde… - ACS …, 2023 - ACS Publications
Within this Perspective, we critically reflect on the role of first-principles molecular dynamics
(MD) simulations in unraveling the catalytic function within zeolites under operating …

DeepQMC: An open-source software suite for variational optimization of deep-learning molecular wave functions

Z Schätzle, PB Szabó, M Mezera… - The Journal of …, 2023 - pubs.aip.org
Computing accurate yet efficient approximations to the solutions of the electronic
Schrödinger equation has been a paramount challenge of computational chemistry for …

Nonadiabatic coupling in trajectory surface hopping: accurate time derivative couplings by the curvature-driven approximation

X Zhao, ICD Merritt, R Lei, Y Shu… - Journal of Chemical …, 2023 - ACS Publications
Trajectory surface hopping (TSH) is a widely used mixed quantum-classical dynamics
method that is used to simulate molecular dynamics with multiple electronic states. In TSH …

Nonempirical range-separated hybrid functional with spatially dependent screened exchange

J Zhan, M Govoni, G Galli - Journal of Chemical Theory and …, 2023 - ACS Publications
Electronic structure calculations based on density functional theory (DFT) have successfully
predicted numerous ground-state properties of a variety of molecules and materials …