The development and applications of multidimensional biomolecular spectroscopy illustrated by photosynthetic light harvesting

GR Fleming, GD Scholes - Quarterly Reviews of Biophysics, 2024 - cambridge.org
The parallel and synergistic developments of atomic resolution structural information, new
spectroscopic methods, their underpinning formalism, and the application of sophisticated …

Ultrafast anisotropy decay reveals structure and energy transfer in supramolecular aggregates

V Erić, JL Castro, X Li, L Dsouza… - The Journal of …, 2023 - ACS Publications
Chlorosomes from green bacteria perform the most efficient light capture and energy
transfer, as observed among natural light-harvesting antennae. Hence, their unique …

Manifestation of hydrogen bonding and exciton delocalization on the absorption and two-dimensional electronic spectra of chlorosomes

V Eric, X Li, L Dsouza, SK Frehan… - The Journal of …, 2023 - ACS Publications
Chlorosomes are supramolecular aggregates that contain thousands of bacteriochlorophyll
molecules. They perform the most efficient ultrafast excitation energy transfer of all natural …

Photon Energy-Dependent Ultrafast Exciton Transfer in Chlorosomes of Chlorobium tepidum and the Role of Supramolecular Dynamics

SK Frehan, L Dsouza, X Li, V Eríc… - The Journal of …, 2023 - ACS Publications
The antenna complex of green sulfur bacteria, the chlorosome, is one of the most efficient
supramolecular systems for efficient long-range exciton transfer in nature. Femtosecond …

Accuracy of approximate methods for the calculation of absorption-type linear spectra with a complex system–bath coupling

JA Nöthling, T Mančal, TPJ Krüger - The Journal of Chemical Physics, 2022 - pubs.aip.org
The accuracy of approximate methods for calculating linear optical spectra depends on
many variables. In this study, we fix most of these parameters to typical values found in …

Observation of Dark States in Two-Dimensional Electronic Spectra of Chlorosomes

V Erić, X Li, L Dsouza, A Huijser… - The Journal of …, 2024 - ACS Publications
Observations of low-lying dark states in several photosynthetic complexes challenge our
understanding of the mechanisms behind their efficient energy transfer processes …

Exploring disordered exciton landscapes in chlorosomes: a quest for spectral signatures

V Eric - 2024 - research.rug.nl
Photosynthesis is a process which involves the conversion of energy coming from sunlight to
energy that serves as a powerhouse for life on Earth. The photosynthetic world is large and …

Modelling of plant light-harvesting spectra

JA Nöthling - 2022 - search.proquest.com
In plants, the life-sustaining process of photosynthesis begins when molecular
lightharvesting complexes capture sunlight. In order to understand the role and function of …

[PDF][PDF] ansen, TLC, Mul, G.,… Hui ser,.(2023)

SK Frehan, L D'Souza, X Li… - … exciton transfer in … - scholarlypublications …
The antenna complex of green sulfur bacteria, the chlorosome, is one of the most efficient
supramolecular systems for efficient long-range exciton transfer in nature. Femtosecond …