Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Gas diffusion electrodes and membranes for CO2 reduction electrolysers

EW Lees, BAW Mowbray, FGL Parlane… - Nature Reviews …, 2022 - nature.com
The CO2 reduction reaction (CO2RR) is a potential means of using renewable electricity to
synthesize commodity chemicals and fuels. The CO2RR can be performed at industrially …

Electroreduction of CO2: Advances in the Continuous Production of Formic Acid and Formate

K Fernández-Caso, G Díaz-Sainz… - ACS Energy …, 2023 - ACS Publications
The study of the electrochemical CO2 reduction to obtain formate (HCOO–) or formic acid
(HCOOH) is receiving much attention as a promising technology. Since continuous–mode …

Localized Alkaline Environment via In Situ Electrostatic Confinement for Enhanced CO2-to-Ethylene Conversion in Neutral Medium

Z Wang, Y Li, X Zhao, S Chen, Q Nian… - Journal of the …, 2023 - ACS Publications
Electrocatalytic CO2 reduction reaction (CO2RR) is one of the most promising routes to
facilitate carbon neutrality. An alkaline electrolyte is typically needed to promote the …

Engineering the NiNC Catalyst Microenvironment Enabling CO2 Electroreduction with Nearly 100% CO Selectivity in Acid

X Sheng, W Ge, H Jiang, C Li - Advanced Materials, 2022 - Wiley Online Library
CO2 electrolysis in acid has emerged as a promising route to achieve high CO2 utilization
due to the inhibition of undesired carbonate formation that generally occurs in alkaline or …

Microenvironment Engineering for the Electrocatalytic CO2 Reduction Reaction

JJ Lv, R Yin, L Zhou, J Li, R Kikas, T Xu… - Angewandte …, 2022 - Wiley Online Library
Rather than just focusing on the catalyst itself in the electrocatalytic CO2 reduction reaction
(eCO2RR), as previously reviewed elsewhere, we herein extend the discussion to the …

Recent Advances in Electrochemical, Photochemical, and Photoelectrochemical Reduction of CO2 to C2+ Products

GH Han, J Bang, G Park, S Choe, YJ Jang, HW Jang… - Small, 2023 - Wiley Online Library
Environmental problems such as global warming are one of the most prominent global
challenges. Researchers are investigating various methods for decreasing CO2 emissions …

Uniting biological and chemical strategies for selective CO2 reduction

HS Shafaat, JY Yang - Nature Catalysis, 2021 - nature.com
The electrochemical reduction of CO2 into useful fuels and chemical feedstocks offers great
promise for conversion to a carbon-neutral economy. However, challenges in product …

Tailoring the Catalytic Microenvironment of Cu2O with SiO2 to Enhance C2+ Product Selectivity in CO2 Electroreduction

T Zhao, J Li, J Liu, F Liu, K Xu, M Yu, W Xu… - ACS Catalysis, 2023 - ACS Publications
Achieving high activity and selectivity of multicarbon products in the CO2 reduction reaction
(CO2RR) on Cu-based electrocatalysts remains challenging due to the limited concentration …

Vitamin C-induced CO2 capture enables high-rate ethylene production in CO2 electroreduction

J Kim, T Lee, HD Jung, M Kim, J Eo, B Kang… - Nature …, 2024 - nature.com
High-rate production of multicarbon chemicals via the electrochemical CO2 reduction can be
achieved by efficient CO2 mass transport. A key challenge for C− C coupling in high-current …