Insights into low thermal conductivity in inorganic materials for thermoelectrics

T Ghosh, M Dutta, D Sarkar… - Journal of the American …, 2022 - ACS Publications
Efficient manipulation of thermal conductivity and fundamental understanding of the
microscopic mechanisms of phonon scattering in crystalline solids are crucial to achieve …

Polar metals: principles and prospects

S Bhowal, NA Spaldin - Annual Review of Materials Research, 2023 - annualreviews.org
We review the class of materials known as polar metals, in which polarity and metallicity
coexist in the same phase. While the notion of polar metals was first invoked more than 50 …

Observation of interplay between phonon chirality and electronic band topology

FGG Hernandez, A Baydin, S Chaudhary, F Tay… - Science …, 2023 - science.org
The recently demonstrated chiral modes of lattice motion carry angular momentum and
therefore directly couple to magnetic fields. Notably, their magnetic moments are predicted …

Engineering ferroelectric instability to achieve ultralow thermal conductivity and high thermoelectric performance in Sn 1− x Ge x Te

A Banik, T Ghosh, R Arora, M Dutta, J Pandey… - Energy & …, 2019 - pubs.rsc.org
High thermoelectric performance of a crystalline solid requires it to have low thermal
conductivity which is one of the utmost material challenges. Herein, we demonstrate how the …

Phonon collapse and second-order phase transition in thermoelectric SnSe

U Aseginolaza, R Bianco, L Monacelli, L Paulatto… - Physical review …, 2019 - APS
Since 2014 the layered semiconductor SnSe in the high-temperature C mcm phase is
known to be the most efficient intrinsic thermoelectric material. Making use of first-principles …

Intrinsically ultralow thermal conductive inorganic solids for high thermoelectric performance

M Dutta, D Sarkar, K Biswas - Chemical Communications, 2021 - pubs.rsc.org
Thermoelectric materials which can convert heat energy to electricity rely on crystalline
inorganic solid state compounds exhibiting low phonon transport (ie low thermal …

Revealing a distortive polar order buried in the Fermi sea

J Shi, W You, X Li, FY Gao, X Peng, S Zhang, J Li… - Science …, 2024 - science.org
Polar metals are challenging to identify spectroscopically because the fingerprints of electric
polarization are often obscured by the presence of screening charges. Here, we unravel …

Strong anharmonicity in the phonon spectra of PbTe and SnTe from first principles

GAS Ribeiro, L Paulatto, R Bianco, I Errea, F Mauri… - Physical Review B, 2018 - APS
At room temperature, PbTe and SnTe are efficient thermoelectrics with a cubic structure. At
low temperature, SnTe undergoes a ferroelectric transition with a critical temperature …

Uncovering the phonon spectra and lattice dynamics of plastically deformable InSe van der Waals crystals

J Wu, Y Lin, M Shu, Y Liu, Y Ma, G Lin, C Zhang… - Nature …, 2024 - nature.com
Abstract Stacking two-dimensional (2D) van der Waals (vdW) materials in a layered bulk
structure provides an appealing platform for the emergence of exotic physical properties. As …

High-resolution inelastic X-ray scattering I: Context, spectrometers, samples, and superconductors

AQR Baron - Synchrotron Light Sources and Free-Electron Lasers …, 2020 - Springer
This chapter reviews nonresonant, meV-resolution inelastic x-ray scattering (IXS), as applied
to the measurement of atomic dynamics of crystalline materials. It, in conjunction with a …