The doublet-spin nature of radical emitters is advantageous for applications in organic light-
emitting diodes, as it avoids the formation of triplet excitons that limit the …

Covalent dimers, particularly pentacenes, are the dominant platform for developing a
mechanistic understanding of intramolecular singlet fission (iSF). Numerous studies have …

Singlet fission in organic semiconductors causes a singlet exciton to decay into a pair of
triplet excitons and holds potential for increasing the efficiency of photovoltaic devices. In …

Organic light-emitting diodes (OLEDs) with doublet-spin radical emitters have emerged as a
new route to efficient display technologies. In contrast to standard organic semiconductors …

Quantum interference (QI)—the constructive or destructive interference of conduction
pathways through molecular orbitals—plays a fundamental role in enhancing or …

High-spin molecules allow for bottom-up qubit design and are promising platforms for
magnetic sensing and quantum information science. Optical addressability of molecular …

We investigate triplet pair dynamics in pentacene dimers that have varying degrees of
coplanarity (pentacene–pentacene twist angle). The fine-tuning of the twist angle was …

The functional properties of organic semiconductors are defined by the interplay between
optically bright and dark states. Organic devices require rapid conversion between these …

Radical emitters have attracted considerable interest because of their potential to surpass
the limitations of singlet emitters due to spin statistics, thereby revolutionizing organic LEDs …

Interchromophoric interactions such as Coulombic coupling and exchange interactions are
crucial to the functional properties of numerous π-conjugated systems. Here, we use …