Time-resolved photoelectron spectroscopy: the continuing evolution of a mature technique
MS Schuurman, V Blanchet - Physical Chemistry Chemical Physics, 2022 - pubs.rsc.org
Time-resolved photoelectron spectroscopy (TRPES) has become one of the most
widespread techniques for probing nonadiabatic dynamics in the excited electronic states of …
widespread techniques for probing nonadiabatic dynamics in the excited electronic states of …
Ultrafast X-ray probes of elementary molecular events
Elementary events that determine photochemical outcomes and molecular functionalities
happen on the femtosecond and subfemtosecond timescales. Among the most ubiquitous …
happen on the femtosecond and subfemtosecond timescales. Among the most ubiquitous …
Conical intersection passages of molecules probed by X-ray diffraction and stimulated Raman spectroscopy
Conical intersections (CoIns) play an important role in ultrafast relaxation channels. Their
monitoring remains a formidable experimental challenge. We theoretically compare the …
monitoring remains a formidable experimental challenge. We theoretically compare the …
Formation of electronic coherences in conical intersection-mediated dynamics
SP Neville, A Stolow… - Journal of Physics B …, 2022 - iopscience.iop.org
We consider the formation of vibrationally-induced transient electronic coherences driven by
conical intersection (CI)-mediated population transfer between two electronic states. By …
conical intersection (CI)-mediated population transfer between two electronic states. By …
Monitoring molecular vibronic coherences in a bichromophoric molecule by ultrafast X-ray spectroscopy
The role of quantum-mechanical coherences in the elementary photophysics of functional
optoelectronic molecular materials is currently under active study. Designing and controlling …
optoelectronic molecular materials is currently under active study. Designing and controlling …
Coherent electronic-vibrational dynamics in deuterium bromide probed via attosecond transient-absorption spectroscopy
Ultrafast laser excitation can trigger complex coherent dynamics in molecules. Here, we
report attosecond transient-absorption experiments addressing simultaneous probing of …
report attosecond transient-absorption experiments addressing simultaneous probing of …
Trends in angle-resolved molecular photoelectron spectroscopy
D Dowek, P Decleva - Physical Chemistry Chemical Physics, 2022 - pubs.rsc.org
The field of angle-resolved molecular photoelectron spectroscopy is reviewed, with
emphasis on foundations and most recent applications in different regimes of light–matter …
emphasis on foundations and most recent applications in different regimes of light–matter …
Towards molecular frame photoelectron angular distributions in polyatomic molecules from lab frame coherent rotational wavepacket evolution
A theory and method for a matrix-based reconstruction of molecular frame (MF)
photoelectron angular distributions (MFPADs) from laboratory frame (LF) measurements …
photoelectron angular distributions (MFPADs) from laboratory frame (LF) measurements …
Ultrafast molecular frame quantum tomography
L Morrigan, SP Neville, M Gregory, AE Boguslavskiy… - Physical review …, 2023 - APS
We develop and experimentally demonstrate a methodology for a full molecular frame
quantum tomography (MFQT) of dynamical polyatomic systems. We exemplify this approach …
quantum tomography (MFQT) of dynamical polyatomic systems. We exemplify this approach …
Resolving multiphoton processes with high-order anisotropy ultrafast X-ray scattering
We present the first results on experimentally measured ultrafast X-ray scattering of strongly
driven molecular iodine and analysis of high-order anisotropic components of the scattering …
driven molecular iodine and analysis of high-order anisotropic components of the scattering …