Search for new physics with atoms and molecules

MS Safronova, D Budker, D DeMille, DFJ Kimball… - Reviews of Modern …, 2018 - APS
This article reviews recent developments in tests of fundamental physics using atoms and
molecules, including the subjects of parity violation, searches for permanent electric dipole …

The search for variation of fundamental constants with clocks

MS Safronova - Annalen der Physik, 2019 - Wiley Online Library
In many theories beyond the Standard Model the quantities that we call “fundamental
constants” become space‐time dependent, leading to corresponding variation of atomic and …

Absolute frequency metrology of buffer-gas-cooled molecular spectra at 1 kHz accuracy level

R Aiello, V Di Sarno, MG Delli Santi, M De Rosa… - Nature …, 2022 - nature.com
By reducing both the internal and translational temperature of any species down to a few
kelvins, the buffer-gas-cooling (BGC) technique has the potential to dramatically improve the …

Quantum cascade laser based hybrid dual comb spectrometer

L Consolino, M Nafa, M De Regis, F Cappelli… - Communications …, 2020 - nature.com
Four-wave-mixing-based quantum cascade laser frequency combs (QCL-FC) are a powerful
photonic tool, driving a recent revolution in major molecular fingerprint regions, ie mid-and …

Optical–optical double-resonance absorption spectroscopy of molecules with kilohertz accuracy

CL Hu, VI Perevalov, CF Cheng, TP Hua… - The Journal of …, 2020 - ACS Publications
Selective pumping and probing of highly excited states of molecules are essential in various
studies but are also challenging because of high density of states, weak transition moments …

Comb-assisted cavity ring-down spectroscopy of a buffer-gas-cooled molecular beam

L Santamaria, V Di Sarno, P De Natale… - Physical Chemistry …, 2016 - pubs.rsc.org
We demonstrate continuous-wave cavity ring-down spectroscopy of a partially
hydrodynamic molecular beam emerging from a buffer-gas-cooling source. Specifically, the …

Narrow-linewidth quantum cascade laser at 8.6 μm

E Fasci, N Coluccelli, M Cassinerio, A Gambetta… - Optics letters, 2014 - opg.optica.org
We report on a narrow-linewidth distributed-feedback quantum cascade laser at 8.6 μm that
is optical-feedback locked to a high-finesse V-shaped cavity. The spectral purity of the …

Optimized cell geometry for buffer-gas-cooled molecular-beam sources

V Singh, AK Samanta, N Roth, D Gusa… - Physical Review A, 2018 - APS
We have designed, constructed, and commissioned a cryogenic helium buffer-gas source
for producing a cryogenically cooled molecular beam and evaluated the effect of different …

Sub-kilohertz linewidth narrowing of a mid-infrared optical parametric oscillator idler frequency by direct cavity stabilization

I Ricciardi, S Mosca, M Parisi, P Maddaloni… - Optics Letters, 2015 - opg.optica.org
We stabilize the idler frequency of a singly resonant optical parametric oscillator directly to
the resonance of a mid-infrared Fabry–Perot reference cavity. This is accomplished by the …

Absolute frequency measurements of CHF3 Doppler-free ro-vibrational transitions at 8.6  μm

A Gambetta, E Vicentini, Y Wang, N Coluccelli… - Optics Letters, 2017 - opg.optica.org
We report on absolute measurements of saturated-absorption line-center frequencies of
room-temperature trifluoromethane using a quantum cascade laser at 8.6 μm and the …