Nonlinear optical signals and spectroscopy with quantum light

KE Dorfman, F Schlawin, S Mukamel - Reviews of Modern Physics, 2016 - APS
Conventional nonlinear spectroscopy uses classical light to detect matter properties through
the variation of its response with frequencies or time delays. Quantum light opens up new …

Entangled two-photon absorption spectroscopy

F Schlawin, KE Dorfman… - Accounts of chemical …, 2018 - ACS Publications
Conspectus The application of quantum states of light such as entangled photons, for
example, created by parametric down conversion, has experienced tremendous progress in …

Single-photon absorption and emission from a natural photosynthetic complex

Q Li, K Orcutt, RL Cook, J Sabines-Chesterking… - Nature, 2023 - nature.com
Photosynthesis is generally assumed to be initiated by a single photon,–from the Sun,
which, as a weak light source, delivers at most a few tens of photons per nanometre squared …

Multidimensional attosecond resonant X-ray spectroscopy of molecules: Lessons from the optical regime

S Mukamel, D Healion, Y Zhang… - Annual review of …, 2013 - annualreviews.org
New free-electron laser and high-harmonic generation X-ray light sources are capable of
supplying pulses short and intense enough to perform resonant nonlinear time-resolved …

Measurements of entangled two-photon absorption in organic molecules with CW-pumped type-I spontaneous parametric down-conversion

JP Villabona-Monsalve, RK Burdick… - The Journal of …, 2020 - ACS Publications
Entangled photons exhibit strong nonclassical frequency and time correlations
simultaneously, which allow them to excite and extract information about molecules in new …

Optically excited entangled states in organic molecules illuminate the dark

L Upton, M Harpham, O Suzer, M Richter… - The Journal of …, 2013 - ACS Publications
We utilize quantum entangled photons to carry out nonlinear optical spectroscopy in organic
molecules with an extremely small number of photons. For the first time, fluorescence is …

Entangled light–matter interactions and spectroscopy

S Szoke, H Liu, BP Hickam, M He… - Journal of Materials …, 2020 - pubs.rsc.org
Entangled photons exhibit non-classical light–matter interactions that create new
opportunities in materials and molecular science. Notably, in entangled two-photon …

Entangled photon spectroscopy

F Schlawin - Journal of Physics B: Atomic, Molecular and Optical …, 2017 - iopscience.iop.org
This tutorial outlines the theory of nonlinear spectroscopy with quantum light, and in
particular with entangled photons. To this end, we briefly review molecular quantum …

Suppression of population transport and control of exciton distributions by entangled photons

F Schlawin, KE Dorfman, BP Fingerhut… - Nature …, 2013 - nature.com
Entangled photons provide an important tool for secure quantum communication, computing
and lithography. Low intensity requirements for multi-photon processes make them idealy …

Efficient modeling of organic chromophores for entangled two-photon absorption

G Kang, K Nasiri Avanaki, MA Mosquera… - Journal of the …, 2020 - ACS Publications
The use of a nonclassical light source for studying molecular electronic structure has been of
great interest in many applications. Here we report a theoretical study of entangled two …