Molecular spins for quantum information technologies

F Troiani, M Affronte - Chemical Society Reviews, 2011 - pubs.rsc.org
Technological challenges for quantum information technologies lead us to consider aspects
of molecular magnetism in a radically new perspective. The design of new derivatives and …

Single-molecule nanomagnets

JR Friedman, MP Sarachik - Annu. Rev. Condens. Matter Phys., 2010 - annualreviews.org
Single-molecule magnets straddle the classical and quantum mechanical worlds, displaying
many fascinating phenomena. They may have important technological applications in …

Coherent terahertz control of antiferromagnetic spin waves

T Kampfrath, A Sell, G Klatt, A Pashkin, S Mährlein… - Nature …, 2011 - nature.com
Ultrafast charge and spin excitations in the elusive terahertz regime, of the electromagnetic
spectrum play a pivotal role in condensed matter,,,,,,,,,,. The electric field of free-space …

Room temperature quantum coherence in a potential molecular qubit

K Bader, D Dengler, S Lenz, B Endeward… - Nature …, 2014 - nature.com
The successful development of a quantum computer would change the world, and current
internet encryption methods would cease to function. However, no working quantum …

Toward molecular 4f single-ion magnet qubits

KS Pedersen, AM Ariciu, S McAdams… - Journal of the …, 2016 - ACS Publications
Quantum coherence is detected in the 4f single-ion magnet (SIM) Yb (trensal), by isotope
selective pulsed EPR spectroscopy on an oriented single crystal. At X-band, the spin–lattice …

Long-lived electronic spin qubits in single-walled carbon nanotubes

JS Chen, KJ Trerayapiwat, L Sun, MD Krzyaniak… - Nature …, 2023 - nature.com
Electron spins in solid-state systems offer the promise of spin-based information processing
devices. Single-walled carbon nanotubes (SWCNTs), an all-carbon one-dimensional …

Strong spin–phonon coupling between a single-molecule magnet and a carbon nanotube nanoelectromechanical system

M Ganzhorn, S Klyatskaya, M Ruben… - Nature …, 2013 - nature.com
Magnetic relaxation processes were first discussed for a crystal of paramagnetic transition
ions. It was suggested that mechanical vibrations of the crystal lattice (phonons) modulate …

A Heterometallic Porphyrin Dimer as a Potential Quantum Gate: Magneto‐Structural Correlations and Spin Coherence Properties

D Ranieri, A Privitera, F Santanni… - Angewandte …, 2023 - Wiley Online Library
In the development of two‐qubit quantum gates, precise control over the intramolecular spin‐
spin interaction between molecular spin units plays a pivotal role. A weak but measurable …

Forging solid-state qubit design principles in a molecular furnace

MJ Graham, JM Zadrozny, MS Fataftah… - Chemistry of …, 2017 - ACS Publications
The realization of quantum information processing would disrupt the status quo in the realm
of computation; the extraordinary power of a hypothetical quantum computer motivates …

Trigonal Bipyramidal V3+ Complex as an Optically Addressable Molecular Qubit Candidate

MS Fataftah, SL Bayliss, DW Laorenza… - Journal of the …, 2020 - ACS Publications
Synthetic chemistry enables a bottom-up approach to quantum information science, where
atoms can be deterministically positioned in a quantum bit or qubit. Two key requirements to …