Experimental Insights into Quantum Spin Ice Physics in Dipole–Octupole Pyrochlore Magnets

EM Smith, E Lhotel, S Petit… - Annual Review of …, 2024 - annualreviews.org
We review a key subset of the experimental studies that have recently focused on cubic
pyrochlore magnets whose pseudospin-1 2 degrees of freedom have mixed dipolar and …

Crystalline Electric-Field Randomness in the Triangular Lattice Spin-Liquid

Y Li, D Adroja, RI Bewley, D Voneshen, AA Tsirlin… - Physical review …, 2017 - APS
We apply moderate-high-energy inelastic neutron scattering (INS) measurements to
investigate Yb 3+ crystalline electric field (CEF) levels in the triangular spin-liquid candidate …

Crystal-field states and defect levels in candidate quantum spin ice

V Porée, E Lhotel, S Petit, A Krajewska, P Puphal… - Physical Review …, 2022 - APS
We report the synthesis of powder and single-crystal samples of cerium pyrohafnate and
their characterization using neutron diffraction, thermogravimetry and x-ray absorption …

Review on crystal structures and magnetic properties of RTX 3 materials

BK Rai, P O'Rourke, UN Roy - Journal of Physics: Condensed …, 2022 - iopscience.iop.org
The structural and compositional diversity of the RTX 3 family of materials offers various
magnetic and thermodynamic properties such as complex magnetic structure, vibronic …

Crystal-field parameters of the rare-earth pyrochlores (, Dy, and Ho)

M Ruminy, E Pomjakushina, K Iida, K Kamazawa… - Physical Review B, 2016 - APS
In this work, we present inelastic neutron scattering experiments which probe the single ion
ground states of the rare-earth pyrochlores R 2 Ti 2 O 7 (R= Tb, Dy, Ho). Dy 2 Ti 2 O 7 and …

Magnetoelastic hybrid excitations in CeAuAl3

P Čermák, A Schneidewind, B Liu… - Proceedings of the …, 2019 - National Acad Sciences
Nearly a century of research has established the Born–Oppenheimer approximation as a
cornerstone of condensed-matter systems, stating that the motion of the atomic nuclei and …

Soft-phonon anomalies and crystal electric field–phonon coupling in cubic lanthanide sesquioxides and

JE Slimak, A Cote, GJ MacDougall, SL Cooper - Physical Review B, 2023 - APS
Phonon softening is a common identifier of strong coupling between electronic and
vibrational degrees of freedom in materials, which is responsible for many of the exotic …

Neutron spectroscopic study of crystal-field excitations and the effect of the crystal field on dipolar magnetism in (, Ho, Er, Tm, and Yb)

P Babkevich, A Finco, M Jeong, B Dalla Piazza… - Physical Review B, 2015 - APS
We present a systematic study of the crystal-field interactions in the Li RF 4 (R= Gd, Ho, Er,
Tm, and Yb) family of rare-earth magnets. Using detailed inelastic neutron scattering …

Magnetoelastically induced vibronic bound state in the spin-ice pyrochlore

J Gaudet, AM Hallas, CRC Buhariwalla, G Sala… - Physical Review B, 2018 - APS
The single-ion physics of Ho 2 Ti 2 O 7 is well understood to produce strong Ising
anisotropy, which is an essential ingredient to its low-temperature spin-ice state. We present …

Mesoscale interplay between phonons and crystal electric field excitations in quantum spin liquid candidate CsYbSe 2

YY Pai, CE Marvinney, L Liang, J Xing… - Journal of Materials …, 2022 - pubs.rsc.org
CsYbSe2, a recently identified quantum spin liquid (QSL) candidate, exhibits strong crystal
electric field (CEF) excitations. Here, we identify phonon and CEF modes with Raman …