Large scale purification in semiconductors using Rydberg excitons

M Bergen, V Walther, B Panda, M Harati… - Nature …, 2023 - nature.com
Improving the quantum coherence of solid-state systems is a decisive factor in realizing solid-
state quantum technologies. The key to optimize quantum coherence lies in reducing the …

Rydberg excitons in Cu2O microcrystals grown on a silicon platform

S Steinhauer, MAM Versteegh, S Gyger… - Communications …, 2020 - nature.com
Cuprous oxide (Cu2O) is a semiconductor with large exciton binding energy and significant
technological importance in applications such as photovoltaics and solar water splitting. It is …

Rydberg excitons in synthetic cuprous oxide

SA Lynch, C Hodges, S Mandal, W Langbein… - Physical Review …, 2021 - APS
High-lying Rydberg states of Mott-Wannier excitons are receiving considerable interest due
to the possibility of adding long-range interactions to the physics of excitons. Here, we study …

Atomistic determination of the surface structure of Cu 2 O (111): Experiment and theory

R Zhang, L Li, L Frazer, KB Chang… - Physical Chemistry …, 2018 - pubs.rsc.org
Cuprous oxide (Cu2O) is a promising catalyst for several important reactions. However, the
atomic structures of defective Cu2O surfaces, which critically affect the catalytic properties …

Photoluminescence spectroscopy of cuprous oxide: Bulk crystal versus crystalline films

M Soltanmohammadi, E Spurio… - … status solidi (a), 2023 - Wiley Online Library
Cuprous oxide (Cu2O) crystals and films of 10–65 nm thickness are investigated via electron
diffraction, scanning tunneling microscopy (STM), and photoluminescence (PL) …

High-resolution nanosecond spectroscopy of even-parity Rydberg excitons in

JP Rogers, LAP Gallagher, D Pizzey, JD Pritchett… - Physical Review B, 2022 - APS
We present a study of even-parity Rydberg exciton states in cuprous oxide using second
harmonic generation (SHG) spectroscopy. Excitonic states with principal quantum number …

Tuning defects in Cu 2 O nanostructures via room temperature mechanical pressing: impacts on defect-dependent optical and photoelectrochemical sensing …

Y Cai, W Zhou, H Wang, J Bi, F Yu, J Fang… - Journal of Materials …, 2024 - pubs.rsc.org
The optical and photoelectrochemical (PEC) sensing performances of transition metal
oxides are greatly dependent on structural defects. However, defect engineering under …

Photoluminescence Characteristics of Post-annealed Cu2O Thin Films

CH Chia, SH Su, YM Hu, JW Chiou, CC Yu… - Journal of Electronic …, 2024 - Springer
Cuprous oxide (Cu 2 O) thin films grown by radio-frequency magnetron sputtering were post-
annealed at 700 C under various oxygen partial pressures (PO 2). Reduction and oxidation …

Taming Charged Defects: Large Scale Purification in Semiconductors using Rydberg Excitons

M Bergen, V Walther, B Panda, M Harati… - arXiv preprint arXiv …, 2023 - arxiv.org
We investigate the interaction between highly excited Rydberg excitons and charged
impurities in the semiconductor Cuprous Oxide. We find that it is long-ranged and based on …

Large-scale characterization of monocrystals via Rydberg excitons

K Morin, D Lagarde, A Gillet, X Marie, T Boulier - Physical Review Materials, 2024 - APS
Rydberg states of excitons can reach microns in size and require extremely pure crystals.
We introduce an experimental method for the rapid and spatially resolved characterization of …