Modern computational studies of the glass transition

L Berthier, DR Reichman - Nature Reviews Physics, 2023 - nature.com
The physics of the glass transition and amorphous materials continues to attract the attention
of a wide research community after decades of effort. Supercooled liquids and glasses have …

Revealing key structural features hidden in liquids and glasses

H Tanaka, H Tong, R Shi, J Russo - Nature Reviews Physics, 2019 - nature.com
A great success of solid state physics comes from the characterization of crystal structures in
the reciprocal (wave vector) space. The power of structural characterization in Fourier space …

Models and algorithms for the next generation of glass transition studies

A Ninarello, L Berthier, D Coslovich - Physical Review X, 2017 - APS
Successful computer studies of glass-forming materials need to overcome both the natural
tendency to structural ordering and the dramatic increase of relaxation times at low …

[HTML][HTML] Configurational entropy of glass-forming liquids

L Berthier, M Ozawa, C Scalliet - The Journal of chemical physics, 2019 - pubs.aip.org
The configurational entropy is one of the most important thermodynamic quantities
characterizing supercooled liquids approaching the glass transition. Despite decades of …

Visualizing slow internal relaxations in a two-dimensional glassy system

Y Chen, Z Ye, K Wang, J Huang, H Tong, Y Jin… - Nature Physics, 2023 - nature.com
Unlike a crystal, a glassy solid state displays slow internal relaxation processes besides
vibrational modes even when structural (α) relaxation is frozen. The precise nature of such …

Configurational entropy measurements in extremely supercooled liquids that break the glass ceiling

L Berthier, P Charbonneau… - Proceedings of the …, 2017 - National Acad Sciences
Liquids relax extremely slowly on approaching the glass state. One explanation is that an
entropy crisis, because of the rarefaction of available states, makes it increasingly arduous …

Hierarchical aging pathways and reversible fragile-to-strong transition upon annealing of a metallic glass former

I Gallino, D Cangialosi, Z Evenson, L Schmitt… - Acta Materialia, 2018 - Elsevier
The change of physical properties during aging and the associated microscopic dynamics of
the Au 49 Cu 26.9 Si 16.3 Ag 5.5 Pd 2.3 bulk metallic glass are investigated using a broad …

A topologically driven glass in ring polymers

D Michieletto, MS Turner - Proceedings of the National …, 2016 - National Acad Sciences
The static and dynamic properties of ring polymers in concentrated solutions remains one of
the last deep unsolved questions in polymer physics. At the same time, the nature of the …

Zero-temperature glass transition in two dimensions

L Berthier, P Charbonneau, A Ninarello… - Nature …, 2019 - nature.com
Liquids cooled towards the glass transition temperature transform into amorphous solids that
have a wide range of applications. While the nature of this transformation is understood …

Size-dependent vitrification in metallic glasses

V Di Lisio, I Gallino, SS Riegler, M Frey… - Nature …, 2023 - nature.com
Reducing the sample size can profoundly impact properties of bulk metallic glasses. Here,
we systematically reduce the length scale of Au and Pt-based metallic glasses and study …