Having served as a playground for fundamental studies on the physics of d and f electrons
for almost a century, magnetic molecules are now becoming increasingly important for …

Vibronic coupling, the interaction between molecular vibrations and electronic states, is a
fundamental effect that profoundly affects chemical processes. In the case of molecular …

Spin-phonon coupling is the main driver of spin relaxation and decoherence in solid-state
semiconductors at finite temperature. Controlling this interaction is a central problem for …

Improving the performance of molecular qubits is a fundamental milestone towards
unleashing the power of molecular magnetism in the second quantum revolution. Taming …

Because of the larger intra-molecular distortion, optical phonons usually have stronger spin-
phonon coupling than acoustic phonons in molecular magnets. This property may pose …

The second quantum revolution harnesses exquisite quantum control for a slate of diverse
applications including sensing, communication, and computation. Of the many candidates …

High-spin molecules allow for bottom-up qubit design and are promising platforms for
magnetic sensing and quantum information science. Optical addressability of molecular …

Electron spin relaxation in paramagnetic transition metal complexes constitutes a key
limitation on the growth of molecular quantum information science. However, there exist very …

Pinpointing vibrational mode contributions to electron spin relaxation (T1) constitutes a key
goal for developing molecular quantum bits (qubits) with long room-temperature coherence …

Paramagnetic molecules offer unique advantages for quantum information science owing to
their spatial compactness, synthetic tunability, room-temperature quantum coherence, and …