Hydrogen and dihydrogen bonds in the reactions of metal hydrides

NV Belkova, LM Epstein, OA Filippov… - Chemical …, 2016 - ACS Publications
The dihydrogen bond an interaction between a transition-metal or main-group hydride (M
H) and a protic hydrogen moiety (H X) is arguably the most intriguing type of hydrogen …

The mechanism of dihydrogen activation by frustrated Lewis pairs revisited

S Grimme, H Kruse, L Goerigk, G Erker - … Chemie International Edition, 2010 - infona.pl
A new picture of H 2 activation is given by state‐of‐the‐art quantum chemical calculations of
potential energy surfaces and transition states and a thorough theoretical analysis. Key …

Rationalizing the Reactivity of Frustrated Lewis Pairs: Thermodynamics of H2 Activation and the Role of Acid−Base Properties

TA Rokob, A Hamza, I Pápai - Journal of the American Chemical …, 2009 - ACS Publications
The acid− base strengths of recently reported frustrated Lewis pairs and their relation with
the thermodynamic feasibility of heterolytic hydrogen splitting reactions are analyzed in …

Dihydrogen bond and X–H… σ interaction as sub‐classes of hydrogen bond

SJ Grabowski - Journal of Physical Organic Chemistry, 2013 - Wiley Online Library
Dihydrogen bond (DHB) and X–H… σ interaction are discussed and compared here. Both
interactions possess numerous characteristics of the hydrogen bond (HB). The Natural Bond …

Reaction of a P/Al‐Based Frustrated Lewis Pair with Ammonia, Borane, and Amine–Boranes: Adduct Formation and Catalytic Dehydrogenation

C Appelt, JC Slootweg… - Angewandte Chemie …, 2013 - Wiley Online Library
The discovery of single-bond activation at transition-metal centers has led to a plethora of
catalytic transformations, which highlights the power of organometallic chemistry. Recently …

Triel bonds, π-hole-π-electrons interactions in complexes of boron and aluminium trihalides and trihydrides with acetylene and ethylene

SJ Grabowski - Molecules, 2015 - mdpi.com
MP2/aug-cc-pVTZ calculations were performed on complexes of aluminium and boron
trihydrides and trihalides with acetylene and ethylene. These complexes are linked through …

Bonding in ammonia borane: An analysis based on the natural orbitals for chemical valence and the extended transition state method (ETS-NOCV)

MP Mitoraj - The Journal of Physical Chemistry A, 2011 - ACS Publications
In the present study the natural orbitals for chemical valence (NOCVs) combined with the
energy decomposition scheme (ETS) were used to characterize bonding in various clusters …

The semiempirical quantum mechanical scoring function for in silico drug design

M Lepšík, J Řezáč, M Kolář, A Pecina, P Hobza… - …, 2013 - Wiley Online Library
This Minireview discusses the latest developments in modern quantum mechanics (QM)‐
based computer‐aided drug design, especially using semiempirical QM (SQM) methods. It …

Tetrel–Hydride Interaction between XH3F (X = C, Si, Ge, Sn) and HM (M = Li, Na, BeH, MgH)

QZ Li, HY Zhuo, HB Li, ZB Liu, WZ Li… - The Journal of Physical …, 2015 - ACS Publications
A tetrel–hydride interaction was predicted and characterized in the complexes of XH3F··· HM
(X= C, Si, Ge, Sn; M= Li, Na, BeH, MgH) at the MP2/aug-cc-pVTZ level, where XH3F and HM …

Structure, energy, vibrational spectrum, and Bader's analysis of π⋯ H hydrogen bonds and H− δ⋯ H+ δ dihydrogen bonds

BG de Oliveira - Physical Chemistry Chemical Physics, 2013 - pubs.rsc.org
In this paper, the intermolecular structural study asserted by the vibrational analysis in the
stretch frequencies of hydrogen bonds (π⋯ H) and dihydrogen bonds (H− δ⋯ H+ δ) have …