High-entropy nanoparticles: Synthesis-structure-property relationships and data-driven discovery

Y Yao, Q Dong, A Brozena, J Luo, J Miao, M Chi… - Science, 2022 - science.org
High-entropy nanoparticles have become a rapidly growing area of research in recent years.
Because of their multielemental compositions and unique high-entropy mixing states (ie …

Operando scanning electrochemical probe microscopy during electrocatalysis

C Santana Santos, BN Jaato, I Sanjuán… - Chemical …, 2023 - ACS Publications
Scanning electrochemical probe microscopy (SEPM) techniques can disclose the local
electrochemical reactivity of interfaces in single-entity and sub-entity studies. Operando …

The new era of high-throughput nanoelectrochemistry

X Xu, D Valavanis, P Ciocci, S Confederat… - Analytical …, 2023 - ACS Publications
To acquire a deeper understanding of electrochemical systems requires techniques that
address nanoscale aspects of electrochemistry, inter alia, the detection and analysis of …

High‐entropy alloy catalysts: from bulk to nano toward highly efficient carbon and nitrogen catalysis

L Yu, K Zeng, C Li, X Lin, H Liu, W Shi, HJ Qiu… - Carbon …, 2022 - Wiley Online Library
High‐entropy alloys (HEAs) have attracted widespread attention as both structural and
functional materials owing to their huge multielement composition space and unique high …

Multiscale analysis of electrocatalytic particle activities: linking nanoscale measurements and ensemble behavior

M Kang, CL Bentley, JT Mefford, WC Chueh… - ACS …, 2023 - ACS Publications
Nanostructured electrocatalysts exhibit variations in electrochemical properties across
different length scales, and the intrinsic catalytic characteristics measured at the nanoscale …

Scalable Synthesis of Multi‐Metal Electrocatalyst Powders and Electrodes and their Application for Oxygen Evolution and Water Splitting

IA Cechanaviciute, RP Antony… - Angewandte Chemie …, 2023 - Wiley Online Library
Multi‐metal electrocatalysts provide nearly unlimited catalytic possibilities arising from
synergistic element interactions. We propose a polymer/metal precursor spraying technique …

[HTML][HTML] Correlative co-located electrochemical multi-microscopy

D Martín-Yerga, PR Unwin, D Valavanis… - Current Opinion in …, 2023 - Elsevier
Correlative co-located electrochemical multi-microscopy is transforming our understanding
of property-function relationships in electrode materials. By coupling scanning …

Evaluating analytical expressions for scanning electrochemical cell microscopy (SECCM)

KL Anderson, MA Edwards - Analytical Chemistry, 2023 - ACS Publications
Scanning electrochemical cell microscopy (SECCM) maps the electrochemical activity of a
surface with nanoscale resolution using an electrolyte-filled nanopipette. The meniscus at …

Discovering High Entropy Alloy Electrocatalysts in Vast Composition Spaces with Multiobjective Optimization

W Xu, E Diesen, T He, K Reuter… - Journal of the American …, 2024 - ACS Publications
High entropy alloys (HEAs) are a highly promising class of materials for electrocatalysis as
their unique active site distributions break the scaling relations that limit the activity of …

Single Entity Electrocatalysis

TB Clarke, LE Krushinski, KJ Vannoy… - Chemical …, 2024 - ACS Publications
Making a measurement over millions of nanoparticles or exposed crystal facets seldom
reports on reactivity of a single nanoparticle or facet, which may depart drastically from …