Deep-ultraviolet nonlinear optical crystals: concept development and materials discovery

L Kang, Z Lin - Light: Science & Applications, 2022 - nature.com
Deep-ultraviolet (DUV, wavelength λ< 200 nm) nonlinear optical (NLO) crystal is the core
component of frequency conversion to generate DUV laser, which plays an important role in …

Emergent deep‐ultraviolet nonlinear optical candidates

M Mutailipu, S Pan - Angewandte Chemie International Edition, 2020 - Wiley Online Library
Advances in the generation of coherent lasers at wavelengths below 200 nm as well as the
associated equipment and technologies have greatly spurred the development of nonlinear …

An excellent deep-ultraviolet birefringent material based on [BO2] infinite chains

F Zhang, X Chen, M Zhang, W Jin, S Han… - Light: Science & …, 2022 - nature.com
Birefringent materials play indispensable roles in modulating the polarization of light and are
vital in the laser science and technology. Currently, the design of birefringent materials …

Double‐Modification Oriented Design of a Deep‐UV Birefringent Crystal Functionalized by [B12O16F4(OH)4] Clusters

C Jin, F Li, B Cheng, H Qiu, Z Yang, S Pan… - Angewandte …, 2022 - Wiley Online Library
Polarization modulation of deep‐UV light is of significance to current technologies, and to
this end, the birefringent crystal has emerged as an invaluable material as it allows for …

Large Second-Harmonic Response and Giant Birefringence of CeF2(SO4) Induced by Highly Polarizable Polyhedra

C Wu, T Wu, X Jiang, Z Wang, H Sha… - Journal of the …, 2021 - ACS Publications
Second-harmonic generation (SHG) response and birefringence are two critically important
properties of nonlinear optical (NLO) materials. However, the simultaneous optimization of …

An interlinked prediction-experiment paradigm discovering deep-ultraviolet fluorooxoborates with desired optical nonlinearity and birefringence

J Zhang, C Wu, H Shi, C Xie, Z Yang, S Pan - Matter, 2023 - cell.com
Exploring new materials that meet urgent needs via advanced paradigms is still a challenge.
Herein, aiming at deep-ultraviolet optical functional materials with targeted properties …

Giant Mid‐Infrared Second‐Harmonic Generation Response in a Densely‐Stacked Van Der Waals Transition‐Metal Oxychloride

C Jin, X Jiang, C Wu, K Duanmu, Z Lin… - Angewandte …, 2023 - Wiley Online Library
Second‐harmonic generation (SHG) is a fundamental optical property of nonlinear optical
(NLO) crystals. Thus far, it has proved difficult to engineer large SHG responses, particularly …

Fluorine‐driven enhancement of birefringence in the fluorooxosulfate: a deep evaluation from a joint experimental and computational study

W Jin, W Zhang, A Tudi, L Wang, X Zhou… - Advanced …, 2021 - Wiley Online Library
Understanding and exploring the functional modules (FMs) consisting of local atomic groups
can promote the development of the materials with functional performances. Oxygen …

Highly Polarizable Hg2+ Induced a Strong Second Harmonic Generation Signal and Large Birefringence in LiHgPO4

BL Wu, CL Hu, FF Mao, RL Tang… - Journal of the American …, 2019 - ACS Publications
A new ultraviolet nonlinear optical material, namely LiHgPO4, was synthesized using the
mild hydrothermal method. The structure of LiHgPO4 features novel double layers …

Toward the enhancement of critical performance for deep-ultraviolet frequency-doubling crystals utilizing covalent tetrahedra

M Mutailipu, Z Yang, S Pan - Accounts of Materials Research, 2021 - ACS Publications
Conspectus Deep-ultraviolet (deep-UV, λ< 200 nm) coherent light is emerging as an
indispensable driving force behind the innovation of optics and materials science. The deep …