Time-resolved measurements of quantum dynamics are based on the availability of
controlled events that are shorter than the typical evolution time scale of the processes to be …

Abstract Coherent anti-Stokes Raman scattering (CARS) with femtosecond laser pulses has
become a widespread method in nonlinear optical spectroscopy and microscopy,. As a third …

As a diagonal projection of the traditional generalized two-dimensional correlation function,
a one-dimensional second-order correlation function in the frequency domain is introduced …

The theory for the application of spectrally tailored ('two color') noisy light in an
interferometric coherent Raman scattering (CRS) experiment called I (2) CRS (3c) is …

Electronic energy transfer in photosynthesis occurs over a range of time scales and under a
variety of intermolecular coupling conditions. Recent work has shown that electronic …

A new technique for measuring the time-and frequency-dependent intensities and phases of
correlation functions of broadband, non–transform-limited (noisy) light is presented. It is …

Based on color-locking noisy field correlation, a time-delayed method is proposed to
suppress the thermal effect, and the ultrafast longitudinal relaxation time can be measured …

Time-resolved IR vibrational spectroscopy has been an invaluable tool for the probing of
intramolecular as well as intermolecular dynamics in the condensed phase. Knowledge …

The theory for temporally multidimensional, electronically resonant four-wave-mixing (FWM)
spectroscopy based on broadband light interferometry is developed. Both homodyne and …

Raman-enhanced polarization beats (REPBs) with broadband noisy light are investigated
using chaotic field, phase-diffusion, and Gaussian-amplitude models. The polarization beat …