Explicitly correlated electrons in molecules

C Hattig, W Klopper, A Kohn, DP Tew - Chemical reviews, 2012 - ACS Publications
One of the central challenges of computational molecular investigation is the solution of the
time-independent, nonrelativistic BornÀ Oppenheimer electronic Schrödinger equation. For …

Electron–molecule collision calculations using the R-matrix method

J Tennyson - Physics Reports, 2010 - Elsevier
The R-matrix method is an embedding procedure which is based on the division of space
into an inner region where the physics is complicated and an outer region for which greatly …

Correlation consistent basis sets for molecular core-valence effects with explicitly correlated wave functions: The atoms B–Ne and Al–Ar

JG Hill, S Mazumder, KA Peterson - The Journal of chemical physics, 2010 - pubs.aip.org
Correlation consistent basis sets have been optimized for accurately describing core-core
and core-valence correlation effects with explicitly correlated F12 methods. The new sets …

Extrapolating MP2 and CCSD explicitly correlated correlation energies to the complete basis set limit with first and second row correlation consistent basis sets

JG Hill, KA Peterson, G Knizia… - The Journal of chemical …, 2009 - pubs.aip.org
Accurate extrapolation to the complete basis set (CBS) limit of valence correlation energies
calculated with explicitly correlated MP2-F12 and CCSD (T)-F12b methods have been …

Local explicitly correlated second-order Møller–Plesset perturbation theory with pair natural orbitals

DP Tew, B Helmich, C Hättig - The Journal of chemical physics, 2011 - pubs.aip.org
We explore using a pair natural orbital analysis of approximate first-order pair functions as
means to truncate the space of both virtual and complementary auxiliary orbitals in the …

Explicitly correlated benchmark calculations on C8H8 isomer energy separations: how accurate are DFT, double-hybrid, and composite ab initio procedures?

A Karton, JML Martin - Molecular Physics, 2012 - Taylor & Francis
Accurate isomerization energies are obtained for a set of 45 C8H8 isomers by means of the
high-level, ab initio W1-F12 thermochemical protocol. The 45 isomers involve a range of …

On the accuracy of explicitly correlated coupled-cluster interaction energies—have orbital results been beaten yet?

K Patkowski - The Journal of Chemical Physics, 2012 - pubs.aip.org
The basis set convergence of weak interaction energies for dimers of noble gases helium
through krypton is studied for six variants of the explicitly correlated, frozen geminal coupled …

Natural transition orbitals for the calculation of correlation and excitation energies

S Höfener, W Klopper - Chemical Physics Letters, 2017 - Elsevier
We propose a scheme to reduce the virtual space in the second-order approximate coupled-
cluster singles-and-doubles (CC2) method, allowing for an accurate description of both …

Explicitly correlated coupled-cluster theory using cusp conditions. I. Perturbation analysis of coupled-cluster singles and doubles (CCSD-F12)

A Köhn, DP Tew - The Journal of chemical physics, 2010 - pubs.aip.org
Geminal functions based on Slater-type correlation factors and fixed expansion coefficients,
determined by cusp conditions, have in recent years been forwarded as an efficient and …

A local pair natural orbital coupled cluster study of Rh catalyzed asymmetric olefin hydrogenation

A Anoop, W Thiel, F Neese - Journal of Chemical Theory and …, 2010 - ACS Publications
The recently developed local pair natural orbital coupled cluster theory with single and
double excitations (LPNO− CCSD) was used to study the rhodium-catalyzed asymmetric …