Exploring the Structural, Dynamic, and Functional Properties of Metal‐Organic Frameworks through Molecular Modeling

F Formalik, K Shi, F Joodaki, X Wang… - Advanced Functional …, 2024 - Wiley Online Library
This review spotlights the role of atomic‐level modeling in research on metal‐organic
frameworks (MOFs), especially the key methodologies of density functional theory (DFT) …

Machine learning the quantum-chemical properties of metal–organic frameworks for accelerated materials discovery

AS Rosen, SM Iyer, D Ray, Z Yao, A Aspuru-Guzik… - Matter, 2021 - cell.com
The modular nature of metal–organic frameworks (MOFs) enables synthetic control over
their physical and chemical properties, but it can be difficult to know which MOFs would be …

Structure–activity relationships that identify metal–organic framework catalysts for methane activation

AS Rosen, JM Notestein, RQ Snurr - Acs Catalysis, 2019 - ACS Publications
In this work, we leverage advances in computational screening based on periodic density
functional theory (DFT) to study a diverse set of experimentally derived metal–organic …

Identifying promising metal–organic frameworks for heterogeneous catalysis via high‐throughput periodic density functional theory

AS Rosen, JM Notestein… - Journal of computational …, 2019 - Wiley Online Library
Metal–organic frameworks (MOFs) are a class of nanoporous materials with highly tunable
structures in terms of both chemical composition and topology. Due to their tunable nature …

Tuning the Redox Activity of Metal–Organic Frameworks for Enhanced, Selective O2 Binding: Design Rules and Ambient Temperature O2 Chemisorption in a Cobalt …

AS Rosen, MR Mian, T Islamoglu, H Chen… - Journal of the …, 2020 - ACS Publications
Metal–organic frameworks (MOFs) with coordinatively unsaturated metal sites are appealing
as adsorbent materials due to their tunable functionality and ability to selectively bind small …

Collective breathing in an eightfold interpenetrated metal–organic framework: from mechanistic understanding towards threshold sensing architectures

K Roztocki, F Formalik, A Krawczuk… - Angewandte Chemie …, 2020 - Wiley Online Library
Functional materials that respond to chemical or physical stimuli through reversible
structural transformations are highly desirable for the integration into devices. Now, a new …

Low-Dimensional Metal–Organic Magnets as a Route toward the S = 2 Haldane Phase

J Pitcairn, A Iliceto, L Cañadillas-Delgado… - Journal of the …, 2023 - ACS Publications
Metal–organic magnets (MOMs), modular magnetic materials where metal atoms are
connected by organic linkers, are promising candidates for next-generation quantum …

Theoretical and Experimental Insights into the Spatial Distribution of Functional Groups in a Multivariate Flexible Metal–Organic Framework

K Roztocki, MK Dudek, M Szufla, F Formalik… - Chemistry of …, 2024 - ACS Publications
Dynamic multicomponent metal–organic frameworks, comprising numerous functional
groups attached to a flexible backbone, expedite the complexity of coordination chemistry …

Predicting band gaps of MOFs on small data by deep transfer learning with data augmentation strategies

Z Zhang, C Zhang, Y Zhang, S Deng, YF Yang, A Su… - RSC …, 2023 - pubs.rsc.org
Porphyrin-based MOFs combine the unique photophysical and electrochemical properties of
metalloporphyrins with the catalytic efficiency of MOF materials, making them an important …

Experimental evidence for vibrational entropy as driving parameter of flexibility in the metal–organic framework ZIF-4 (Zn)

KT Butler, P Vervoorts, MG Ehrenreich… - Chemistry of …, 2019 - ACS Publications
Large structural flexibility in some metal–organic frameworks (MOFs) is not only fascinating
from a fundamental point of view but offers exciting opportunities in the areas of gas sensing …