Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Designing a built-in electric field for efficient energy electrocatalysis

X Zhao, M Liu, Y Wang, Y Xiong, P Yang, J Qin… - ACS …, 2022 - ACS Publications
To utilize intermittent renewable energy as well as achieve the goals of peak carbon dioxide
emissions and carbon neutrality, various electrocatalytic devices have been developed …

Continuous electroproduction of formate via CO2 reduction on local symmetry-broken single-atom catalysts

J Dong, Y Liu, J Pei, H Li, S Ji, L Shi, Y Zhang… - Nature …, 2023 - nature.com
Atomic-level coordination engineering is an efficient strategy for tuning the catalytic
performance of single-atom catalysts (SACs). However, their rational design has so far been …

Gas diffusion electrodes, reactor designs and key metrics of low-temperature CO2 electrolysers

D Wakerley, S Lamaison, J Wicks, A Clemens… - Nature Energy, 2022 - nature.com
CO2 emissions can be recycled via low-temperature CO2 electrolysis to generate products
such as carbon monoxide, ethanol, ethylene, acetic acid, formic acid and propanol. In recent …

Stability Issues in Electrochemical CO2 Reduction: Recent Advances in Fundamental Understanding and Design Strategies

W Lai, Y Qiao, Y Wang, H Huang - Advanced Materials, 2023 - Wiley Online Library
Electrochemical CO2 reduction reaction (CO2RR) offers a promising approach to close the
anthropogenic carbon cycle and store intermittent renewable energy in fuels or chemicals …

Surface passivation for highly active, selective, stable, and scalable CO2 electroreduction

J Zhu, J Li, R Lu, R Yu, S Zhao, C Li, L Lv, L Xia… - Nature …, 2023 - nature.com
Electrochemical conversion of CO2 to formic acid using Bismuth catalysts is one the most
promising pathways for industrialization. However, it is still difficult to achieve high formic …

Electrochemical C–N coupling of CO 2 and nitrogenous small molecules for the electrosynthesis of organonitrogen compounds

X Peng, L Zeng, D Wang, Z Liu, Y Li, Z Li… - Chemical Society …, 2023 - pubs.rsc.org
Electrochemical C–N coupling reactions based on abundant small molecules (such as CO2
and N2) have attracted increasing attention as a new “green synthetic strategy” for the …

Acidic CO2-to-HCOOH electrolysis with industrial-level current on phase engineered tin sulfide

H Shen, H Jin, H Li, H Wang, J Duan, Y Jiao… - Nature …, 2023 - nature.com
Acidic CO2-to-HCOOH electrolysis represents a sustainable route for value-added CO2
transformations. However, competing hydrogen evolution reaction (HER) in acid remains a …

Electroreduction of CO2: Advances in the Continuous Production of Formic Acid and Formate

K Fernández-Caso, G Díaz-Sainz… - ACS Energy …, 2023 - ACS Publications
The study of the electrochemical CO2 reduction to obtain formate (HCOO–) or formic acid
(HCOOH) is receiving much attention as a promising technology. Since continuous–mode …

Copper-catalysed exclusive CO2 to pure formic acid conversion via single-atom alloying

T Zheng, C Liu, C Guo, M Zhang, X Li, Q Jiang… - Nature …, 2021 - nature.com
Converting CO2 emissions, powered by renewable electricity, to produce fuels and
chemicals provides an elegant route towards a carbon-neutral energy cycle. Progress in the …