The viscosity of atmospherically relevant organic particles

JP Reid, AK Bertram, DO Topping, A Laskin… - Nature …, 2018 - nature.com
The importance of organic aerosol particles in the environment has been long established,
influencing cloud formation and lifetime, absorbing and scattering sunlight, affecting …

Predicting the influence of particle size on the glass transition temperature and viscosity of secondary organic material

M Petters, S Kasparoglu - Scientific reports, 2020 - nature.com
Atmospheric aerosols can assume liquid, amorphous semi-solid or glassy, and crystalline
phase states. Particle phase state plays a critical role in understanding and predicting …

Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition

WSW DeRieux, Y Li, P Lin, J Laskin… - Atmospheric …, 2018 - acp.copernicus.org
Secondary organic aerosol (SOA) accounts for a large fraction of submicron particles in the
atmosphere. SOA can occur in amorphous solid or semi-solid phase states depending on …

Humidity-dependent viscosity of secondary organic aerosol from ozonolysis of β-caryophyllene: Measurements, predictions, and implications

AM Maclean, NR Smith, Y Li, Y Huang… - ACS Earth and Space …, 2021 - ACS Publications
To predict important secondary organic aerosol (SOA) properties, information on viscosity or
diffusion rates within SOA is needed. Ozonolysis of β-caryophyllene is an important SOA …

Predicting secondary organic aerosol phase state and viscosity and its effect on multiphase chemistry in a regional-scale air quality model

R Schmedding, QZ Rasool, Y Zhang… - Atmospheric …, 2020 - acp.copernicus.org
Atmospheric aerosols are a significant public health hazard and have substantial impacts on
the climate. Secondary organic aerosols (SOAs) have been shown to phase separate into a …

A predictive group-contribution model for the viscosity of aqueous organic aerosol

NR Gervasi, DO Topping, A Zuend - Atmospheric Chemistry and …, 2020 - acp.copernicus.org
The viscosity of primary and secondary organic aerosol (SOA) has important implications for
the processing of aqueous organic aerosol phases in the atmosphere, their involvement in …

[HTML][HTML] Timescales of secondary organic aerosols to reach equilibrium at various temperatures and relative humidities

Y Li, M Shiraiwa - Atmospheric Chemistry and Physics, 2019 - acp.copernicus.org
Secondary organic aerosols (SOA) account for a substantial fraction of air particulate matter,
and SOA formation is often modeled assuming rapid establishment of gas–particle …

Predictions of diffusion rates of large organic molecules in secondary organic aerosols using the Stokes–Einstein and fractional Stokes–Einstein relations

E Evoy, AM Maclean, G Rovelli, Y Li… - Atmospheric …, 2019 - acp.copernicus.org
Abstract Information on the rate of diffusion of organic molecules within secondary organic
aerosol (SOA) is needed to accurately predict the effects of SOA on climate and air quality …

Direct measurements of semi-volatile organic compound dynamics show near-unity mass accommodation coefficients for diverse aerosols

X Liu, DA Day, JE Krechmer, W Brown… - Communications …, 2019 - nature.com
The partitioning of low-and semi-volatile organic compounds into and out of particles
significantly influences secondary organic aerosol formation and evolution. Most …

Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA

NR Smith, GV Crescenzo, Y Huang… - Environmental …, 2021 - pubs.rsc.org
Molecular composition, viscosity, and liquid–liquid phase separation (LLPS) were
investigated for secondary organic aerosol (SOA) derived from synthetic mixtures of volatile …