In the last few years, there has been a great surge in the interest and activity in the quantum
mechanical description of dynamical processes in large molecular systems. Till very …

This paper in the series gives our full account of the preliminary results reported in a
communication [Cheng, Zhong, and Zewail, J. Chem. Phys. 103, 5153 (1995)] on real‐time …

Time resolved studies of the title reaction have been carried out by photodissociating the HI
moiety within weakly bound CO2–HI complexes. The HOCO° intermediate decomposes via …

The photodissociation of molecules and the interaction of the products with the surrounding
cage atoms is an important field of research in solvation dynamics. The targeted generation …

Center-of-mass translational energy distributions of the dominant primary products resulting
from 193.3 nm excitation of jet-cooled CH30H, CH30D, and CD30H were obtained by using …

A new method for approximate solution of the time-dependent vibrational Schrödinger
equation, applicable to extended molecular systems, is presented. The new method is …

The ultraviolet photolysis of HBr molecules and (HBr) n clusters with average size around
n̄= 9 is studied at three different wavelengths of 243, 205, and 193 nm. Applying polarized …

The study of photochemical reactions in clusters has attracted much interest in recent years.
Aside from the intrinsic interest in such processes, they are considered to provide …

A pulsed-extraction time-of-flight method was employed to investigate the photodissociation
dynamics of the C6H6− I2 charge-transfer state. Measurement of the kinetic energy release …

Investigations of the van der Waals complexes Rg–HX (XF, Cl) 1, 2 using high-resolution
gas phase spectroscopy have been particularly fruitful. Indeed, these species have become …